Synthesis of photoresponsive biobased adhesive polymers via the Passerini three-component reaction

被引：0
|
作者：
Chou, Li-Chieh [1 ]
Matsubara, Kiho [1 ]
Takada, Kenji [2 ]
Kaneko, Tatsuo [2 ]
Kakuchi, Ryohei [1 ]
机构：
[1] Gunma Univ, Fac Sci & Technol, Div Mol Sci, 1-5-1 Tenjin, Kiryu, Gunma 3768515, Japan
[2] Japan Adv Inst Sci & Technol JAIST, Grad Sch Adv Sci & Technol, Sustainable Innovat Res Area, 1-1 Asahidai, Nomi, Ishikawa, Japan
来源：
POLYMER JOURNAL | 2023年 / 55卷 / 10期
关键词：
POLYMERIZATION; ACID; PERFORMANCE; CHEMISTRY; CATECHOL; RESIN;
D O I：
10.1038/s41428-023-00806-4
中图分类号：
O63 [高分子化学（高聚物）];
学科分类号：
070305 ; 080501 ; 081704 ;
摘要：
In this study, adhesive polymers were designed and synthesized using biobased compounds as building blocks. Using the Passerini three-component reaction (Passerini-3CR) as a postpolymerization modification process, photoresponsive phenylpropanoid units were introduced into biobased adhesive polymers via a one-step process that bypassed a protection-deprotection strategy. These biobased adhesive polymers showed good adhesion properties for quartz plates. Photoirradiation affected the adhesion behaviors of the polymers, probably due to the [2 + 2] self-cycloaddition of phenylpropanoid-derived vinyl moieties.
引用
收藏
页码：1067 / 1074
页数：8
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