Most automotive plastic waste (APW) is landfilled or used in energy recovery as it is unsuitable for high-quality product mechanical recycling. Chemical recycling via pyrolysis offers a pathway toward closing the material loop by handling this heterogeneous waste and providing feedstock for producing virgin plastics. This study compares chemical recycling and energy recovery scenarios for APW regarding climate change impact and cumulative energy demand (CED), assessing potential environmental advantages. In addition, an economic assessment is conducted. In contrast to other studies, the assessments are based on pyrolysis experiments conducted with an actual waste fraction. Mass balances and product composition are reported. The experimental data is combined with literature data for up- and downstream processes for the assessment. Chemical recycling shows a lower net climate change impact (0.57 to 0.64 kg CO(2)e/kg waste input) and CED (3.38 to 4.41 MJ/kg waste input) than energy recovery (climate change impact: 1.17 to 1.25 kg CO(2)e/kg waste input; CED: 6.94 to 7.97 MJ/kg waste input), while energy recovery performs better economically (net processing cost of -0.05 to -0.02euro/kg waste input) compared to chemical recycling (0.05 to 0.08euro/kg waste input). However, chemical recycling keeps carbon in the material cycle contributing to a circular economy and reducing the dependence on fossil feedstocks. Therefore, an increasing circularity of APW through chemical recycling shows a conflict between economic and environmental objectives.
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Univ Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Univ Michigan, Michigan Inst Computat Discovery & Engn, Ann Arbor, MI 48109 USAUniv Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Hou, Ping
Xu, Yifan
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Univ Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USAUniv Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Xu, Yifan
Taiebat, Morteza
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Univ Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Univ Michigan, Dept Civil & Environm Engn, Ann Arbor, MI 48109 USAUniv Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Taiebat, Morteza
Lastoskie, Christian
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Univ Michigan, Dept Civil & Environm Engn, Ann Arbor, MI 48109 USAUniv Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Lastoskie, Christian
Miller, Shelie A.
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Univ Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Univ Michigan, Dept Civil & Environm Engn, Ann Arbor, MI 48109 USAUniv Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Miller, Shelie A.
Xu, Ming
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Univ Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
Univ Michigan, Dept Civil & Environm Engn, Ann Arbor, MI 48109 USAUniv Michigan, Sch Environm & Sustainabil, Ann Arbor, MI 48109 USA
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Univ Fed Minas Gerais, Dept Sanit & Environm Engn, Av Antonio Carlos 6627, Belo Horizonte, MG, BrazilUniv Fed Minas Gerais, Dept Sanit & Environm Engn, Av Antonio Carlos 6627, Belo Horizonte, MG, Brazil
de Paula, Eduardo Coutinho
Santos Amaral, Miriam Cristina
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Univ Fed Minas Gerais, Dept Sanit & Environm Engn, Av Antonio Carlos 6627, Belo Horizonte, MG, BrazilUniv Fed Minas Gerais, Dept Sanit & Environm Engn, Av Antonio Carlos 6627, Belo Horizonte, MG, Brazil
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Brunel Univ London, Coll Engn Design & Phys Sci, Heat Pipe & Thermal Management Res Grp, London UB8 3PH, EnglandBrunel Univ London, Coll Engn Design & Phys Sci, Heat Pipe & Thermal Management Res Grp, London UB8 3PH, England
Vlasopoulos, Antonis
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Malinauskaite, Jurgita
Zabnienska-Gora, Alina
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Brunel Univ London, Coll Engn Design & Phys Sci, Heat Pipe & Thermal Management Res Grp, London UB8 3PH, EnglandBrunel Univ London, Coll Engn Design & Phys Sci, Heat Pipe & Thermal Management Res Grp, London UB8 3PH, England
Zabnienska-Gora, Alina
Jouhara, Hussam
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Brunel Univ London, Coll Engn Design & Phys Sci, Heat Pipe & Thermal Management Res Grp, London UB8 3PH, England
Vytautas Magnus Univ, Kaunas, LithuaniaBrunel Univ London, Coll Engn Design & Phys Sci, Heat Pipe & Thermal Management Res Grp, London UB8 3PH, England