Few-Layer Fullerene Network for Photocatalytic Pure Water Splitting into H2 and H2O2

被引：16

作者：

Wang, Taotao ^{[1
,2
]}

Zhang, Li ^{[1
]}

Wu, Jinbao ^{[1
]}

Chen, Muqing ^{[2
]}

Yang, Shangfeng ^{[1
]}

Lu, Yalin ^{[1
]}

Du, Pingwu ^{[1
]}

机构：

[1] Univ Sci & Technol China, Anhui Lab Adv Photon Sci & Technol, Key Lab Precis & Intelligent Chem, Dept Mat Sci & Engn, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China

[2] Dongguan Univ Technol, Sch Mat Sci & Engn, Dongguan 523808, Guangdong, Peoples R China

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2023年 / 62卷 / 40期

基金：

中国国家自然科学基金;

关键词：

Fullerene; Hydrogen; Hydrogen Peroxide; Nanosheet; Solar Water Splitting; CARBON NITRIDE; EVOLUTION; MECHANISM;

D O I：

10.1002/anie.202311352

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A few-layer fullerene network possesses several advantageous characteristics, including a large surface area, abundant active sites, high charge mobility, and an appropriate band gap and band edge for solar water splitting. Herein, we report for the first time that the few-layer fullerene network shows interesting photocatalytic performance in pure water splitting into H-2 and H2O2 in the absence of any sacrificial reagents. Under optimal conditions, the H-2 and H2O2 evolution rates can reach 91 and 116 mu molg(-1)h(-1), respectively, with good stability. This work demonstrates the novel application of the few-layer fullerene network in the field of energy conversion.

引用

页数：5

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