Recycling and Reusing of Graphite from Retired Lithium-ion Batteries: A Review

The proliferation of rechargeable lithium-ion batteries (LIBs) over the past decade has led to a significant increase in the number of electric vehicles (EVs) powered by these batteries reaching the end of their lifespan. With retired EVs becoming more prevalent, recycling and reusing their components, particularly graphite, has become imperative as the world transitions toward electric mobility. Graphite constitutes approximate to 20% of LIBs by weight, making it a valuable resource to be conserved. This review presents an in-depth analysis of the current global graphite mining landscape and explores potential opportunities for the "second life" of graphitefrom depleted LIBs. Various recycling and reactivation technologies in both industry and academia are discussed, along with potential applications for recycled graphite forming a vital aspect of the waste management hierarchy. Furthermore, this review addresses the future challenges faced by the recycling industry in dealing with expired LIBs, encompassing environmental, economic, legal, and regulatory considerations. In conclusion, this review provides a comprehensive overview of the developments in recycling and reusing graphite from retired LIBs, offering valuable insights for forthcoming large-scale recycling efforts. Expired lithium-ion batteries (LIBs) contain valuable battery-grade graphite materials. However, graphite is largely overlooked due to its lower profitability compared to cathode materials. This review discusses the future challenges facing the recycling industry in handling waste graphite and provides a comprehensive overview of the development of graphite recycling and reuse from spent LIBs, offering valuable insights for upcoming large-scale recycling efforts.image