Request for 35Cl(n,p) reaction cross-section measurements and re-evaluations from the standpoint of molten chloride salt fast reactor design

被引:4
|
作者
Tahara, Yoshihisa [1 ,3 ,4 ]
Hirano, Haruka [1 ]
Chiba, Satoshi [1 ,2 ]
Mochizuki, Hiroyasu [1 ]
Katabuchi, Tatsuya [1 ]
机构
[1] Tokyo Inst Technol, Inst Innovat Res, Lab Zero Carbon Energy, Tokyo, Japan
[2] NAT Corp, NAT Res Ctr, Ibaraki, Japan
[3] Tokyo Inst Technol, Inst Innovat Res, Lab Zero Carbon Energy, 2-12-1 Ookayama,Meguro Ku, Tokyo 1528550, Japan
[4] NAIS Co Inc, 416 Muramatsu, Ibaraki, Tokai, Japan
关键词
Molten salt reactor; chloride; fast reactor; transmutation; TRU; Cl-35(n; p); reaction;
D O I
10.1080/00223131.2023.2282553
中图分类号
TL [原子能技术]; O571 [原子核物理学];
学科分类号
0827 ; 082701 ;
摘要
A molten chloride salt fast reactor with inherent safety features is being studied in order to utilize spent fuel discharged from light-water reactors effectively and to reduce environmental burdens. A hard neutron spectrum is required to achieve the transmutation of TRU efficiently, which can be realized by using a molten chloride salt. However, it was found that the criticality analysis shows a large difference of 2%Delta k among the effective multiplication factors (k(eff)) obtained using several evaluated nuclear data libraries. A sensitivity analysis was performed to investigate the cause of the difference in k(eff) and it was clarified that the difference of 2%Delta k/k reactivity was due to the difference in cross sections of the Cl-35(n,p)S-35 reaction. Such a large difference in keff makes a reliable core design difficult and strongly affects important core characteristics such as the TRU transmutation rate, conversion ratio, and so on. Therefore, this paper has been prepared to make a strong request for measurements and re-evaluations of the (n,p) cross section of Cl-35.
引用
收藏
页码:277 / 284
页数:8
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