Recent progress in homogeneous molecular photoredox catalysis towards hydrogen evolution reaction and future perspective

被引:6
|
作者
Mawrie, Ladapborlang [1 ]
Rahman, Fazlur [1 ]
Ali, Md. Ashif [2 ]
Gazi, Sarifuddin [1 ]
机构
[1] Univ Sci & Technol Meghalaya, Sch Appl Sci, Dept Chem, Kling Rd,Baridua 9th Mile, Ri Bhoi 793101, Meghalaya, India
[2] Ramakrishna Miss Residential Coll Autonomous Naren, Dept Chem, Kolkata 700103, W Bengal, India
关键词
Photoredox catalyst; Earth abundant molecular catalysts; Hydrogen production; Homogeneous reaction; Visible light; VISIBLE-LIGHT PHOTOREDOX; METAL-FREE SYSTEM; O BOND-CLEAVAGE; COPPER-BASED PHOTOSENSITIZERS; CARBON EMISSIONS REDUCTION; POROUS ORGANIC FRAMEWORKS; DONOR-ACCEPTOR MOLECULES; C-H ARYLATION; ELECTRON-TRANSFER; WATER REDUCTION;
D O I
10.1016/j.apcata.2022.119010
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The bad impact of fossil fuel and the need of green energy resources have directed many researchers to develop various light-driven, CO2 non emissive hydrogen producing catalytic routes. Majority of such routes involve a catalytic duo made up of a light harvesting photoredox catalyst and a proton reducing catalyst in combination with an excessive amount of sacrificial electron donor. An increasing number of molecular photocatalytic systems for hydrogen evolution reaction (HER) are found in the literature with the progressive turnover frequency (TOF) and turnover number (TON). The development is tip toeing towards the photocatalytic systems with required efficiency and durability for the production of green hydrogen. The present work is focused on conferring the basic understanding of the photoredox process for the generation of molecular hydrogen as green fuel, covering recent important reports available in the literature under homogeneous reaction medium. It also includes the future direction of research and perspective for the economically viable green route of hydrogen production.
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页数:43
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