Bubble-propelled micromotors for ammonia generation

被引:2
|
作者
Campos, Rebeca Ferrer [1 ]
Bachimanchi, Harshith [2 ]
Volpe, Giovanni [2 ]
Villa, Katherine [1 ]
机构
[1] Inst Chem Res Catalonia ICIQ, Av Paisos Catalans 16, E-43007 Tarragona, Spain
[2] Univ Gothenburg, Dept Phys, Origovagen 6B, S-41296 Gothenburg, Sweden
基金
欧洲研究理事会;
关键词
CATALYTIC MICROMOTORS; REMOVAL; LACCASE; POLLUTANTS; UREA;
D O I
10.1039/d3nr03804a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Micromotors have emerged as promising tools for environmental remediation, thanks to their ability to autonomously navigate and perform specific tasks at the microscale. In this study, we present the development of MnO2 tubular micromotors modified with laccase for enhanced oxidation of organic pollutants by providing an additional oxidative catalytic pathway for pollutant removal. These modified micromotors exhibit efficient ammonia generation through the catalytic decomposition of urea, suggesting their potential application in the field of green energy generation. Compared to bare micromotors, the MnO2 micromotors modified with laccase exhibit a 20% increase in rhodamine B degradation. Moreover, the generation of ammonia increased from 2 to 31 ppm in only 15 min, evidencing their high catalytic activity. To enable precise tracking of the micromotors and measurement of their speed, a deep-learning-based tracking system was developed. Overall, this work expands the potential applicability of bio-catalytic tubular micromotors in the energy field. Here, we introduce self-propelled biocatalytic micromotors for simultaneous organic pollutant removal and green energy generation. The study demonstrates remarkable results, showcasing the potential to generate ammonia from wastewater in short time.
引用
收藏
页码:15785 / 15793
页数:9
相关论文
共 50 条
  • [1] Role of Bubble Evolution in the Bubble-Propelled Janus Micromotors
    Chen, Gang
    Wang, Xuekui
    Zhang, Bingyang
    Zhang, Fangfang
    Wang, Zhibin
    Zhang, Baiqiang
    Li, Guopei
    [J]. MICROMACHINES, 2023, 14 (07)
  • [2] Asparaginase immobilized, magnetically guided, and bubble-propelled micromotors
    Evli, Sinem
    Ondes, Baha
    Uygun, Murat
    Uygun, Deniz Aktas
    [J]. PROCESS BIOCHEMISTRY, 2021, 108 : 103 - 109
  • [3] Microfluidic Fabrication of Bubble-Propelled Micromotors for Wastewater Treatment
    Ren, Meng
    Guo, Weilin
    Guo, Huaisu
    Ren, Xiaohua
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2019, 11 (25) : 22761 - 22767
  • [4] Bubble-Propelled Micromotors for Enhanced Transport of Passive Tracers
    Orozco, Jahir
    Jurado-Sanchez, Beatriz
    Wagner, Gregory
    Gao, Wei
    Vazquez-Duhalt, Rafael
    Sattayasamitsathit, Sirilak
    Galarnyk, Michael
    Cortes, Allan
    Saintillan, David
    Wang, Joseph
    [J]. LANGMUIR, 2014, 30 (18) : 5082 - 5087
  • [5] Bubble-propelled trimetallic microcaps as functional catalytic micromotors
    Safdar, M.
    Itkonen, T.
    Janis, J.
    [J]. RSC ADVANCES, 2015, 5 (17): : 13171 - 13174
  • [6] Bubble-Propelled Jellyfish-like Micromotors for DNA Sensing
    Zhang, Xueqing
    Chen, Chengtao
    Wu, Jie
    Ju, Huangxian
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2019, 11 (14) : 13581 - 13588
  • [7] A Viscosity-Based Model for Bubble-Propelled Catalytic Micromotors
    Wang, Zhen
    Chi, Qingjia
    Liu, Lisheng
    Liu, Qiwen
    Bai, Tao
    Wang, Qiang
    [J]. MICROMACHINES, 2017, 8 (07):
  • [8] The gating effect by thousands of bubble-propelled micromotors in macroscale channels
    Teo, Wei Zhe
    Wang, Hong
    Pumera, Martin
    [J]. NANOSCALE, 2015, 7 (27) : 11575 - 11579
  • [9] Bubble-Propelled Hierarchical Porous Micromotors from Evolved Double Emulsions
    Su, Yao-Yao
    Zhang, Mao-Jie
    Wang, Wei
    Deng, Chuan-Fu
    Peng, Jian
    Liu, Zhuang
    Faraj, Yousef
    Ju, Xiao-Jie
    Xie, Rui
    Chu, Liang-Yin
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2019, 58 (04) : 1590 - 1600
  • [10] Integration of BiOI nanosheets into bubble-propelled micromotors for efficient water purification
    Zhou, Huaijuan
    Wu, Bing
    Dekanovsky, Lukas
    Wei, Shuangying
    Khezri, Bahareh
    Hartman, Tomas
    Li, Jinhua
    Sofer, Zdenek
    [J]. FLATCHEM, 2021, 30