Holographic Nano-Imaging of Terahertz Dirac Plasmon Polaritons Topological Insulator Antenna Resonators

被引:5
|
作者
Pistore, Valentino [1 ,2 ]
Viti, Leonardo [1 ,2 ]
Schiattarella, Chiara [1 ,2 ]
Wang, Zhengtianye [3 ]
Law, Stephanie [4 ]
Mitrofanov, Oleg [5 ]
Vitiello, Miriam S. [1 ,2 ]
机构
[1] Ist Nanosci, NEST, CNR, Piazza San Silvestro 12, I-56127 Pisa, Italy
[2] Scuola Normale Super Pisa, Piazza San Silvestro 12, I-56127 Pisa, Italy
[3] Univ Delaware, Dept Mat Sci & Engn, Newark, DE 19716 USA
[4] Penn State Univ, Mat Sci & Engn, University Pk, PA 16802 USA
[5] UCL, Elect & Elect Engn, London WC1E 7JE, England
基金
欧洲研究理事会; 英国工程与自然科学研究理事会;
关键词
large area topological insulators; MBE; near field; plasmon polaritons; SURFACE; BI2SE3; INTERFEROMETRY; STATE; MODES; FILMS;
D O I
10.1002/smll.202308116
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Excitation of Dirac plasmon polaritons (DPPs) in bi-dimensional materials have attracted considerable interest in recent years, both from perspectives of understanding their physics and exploring their transformative potential for nanophotonic devices, including ultra-sensitive plasmonic sensors, ultrafast saturable absorbers, modulators, and switches. Topological insulators (TIs) represent an ideal technological platform in this respect because they can support plasmon polaritons formed by Dirac carriers in the topological surface states. Tracing propagation of DPPs is a very challenging task, particularly at terahertz (THz) frequencies, where the DPP wavelength becomes over one order of magnitude shorter than the free space photon wavelength. Furthermore, severe attenuation hinders the comprehensive analysis of their characteristics. Here, the properties of DPPs in real TI-based devices are revealed. Bi2Se3 rectangular antennas can efficiently confine the propagation of DPPs to a single dimension and, as a result, enhance the DPPs visibility despite the strong intrinsic attenuation. The plasmon dispersion and loss properties from plasmon profiles are experimentally determined, along the antennas, obtained using holographic near-field nano-imaging in a wide range of THz frequencies, from 2.05 to 4.3 THz. The detailed investigation of the unveiled DPP properties can guide the design of novel topological quantum devices exploiting their directional propagation. It is demonstrated that Bi2Se3 rectangular antennas can efficiently confine the propagation of Dirac plasmon polaritons to a single dimension. Plasmon dispersion and loss properties from plasmon profiles are experimentally determined along the antennas by means of holographic near-field nano-imaging in a wide range of THz frequencies, from 2.05 to 4.3 THz.image
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页数:8
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