Effects of smoke on marine low clouds and radiation during 2020 western United States wildfires

Biomass burning aerosols (BBAs) influence the climate directly by scattering and absorbing sunlight and indirectly by changing the cloud properties through serving as cloud condensation nuclei (CCN) or ice-nucleating particles (INPs). Here we used the WRF-Chem model to simulate the transport of BBAs and their interactions with clouds and radiation during the western United States wildfires in September 2020. The simulated cloud and aerosol fields are comparable to the satellite observations from CALIPSO and MODIS. It is shown that smoke exerts negative radiative effects over both ocean and land. Over the nearly cloudless land, the negative radiative effect is caused by aerosols reflecting shortwave radiation. However, over the ocean covered by stratocumulus, aerosol-cloud interaction (ACI) induces a significant negative radiative effect (-25.6 W/m2 on average), because the reduction of droplet radius not only increases the brightness of clouds and prolongs their lifespan, but also cools their surroundings and increases relative humidity, which in turn increases cloud water content. On the contrary, aerosol-radiation interaction (ARI) leads to a positive radiative effect (+10.3 W/m2 on average) over the oceanic regions due to the absorption of sunlight reflected by low clouds and a slight decrease in cloud water. In our research, the counterclockwise vortex over the Northeast Pacific transports the smoke to remote regions and lifts the smoke to 4-8 km height. This results in a wide-ranging impact of the smoke on clouds and radiation, yet it diminishes the magnitude of ARI's effect on marine stratocumulus. Moreover, over ocean, ARI results in cooling at the cloud top and warming close to the sea surface, leading to a rise in marine stratocumulus height. These vertical atmospheric adjustments within the PBL differ from the reduced surface temperature with suppressed PBL over terrestrial regions.