Soot Aerosols from Wheat Stubble Burning Lead to Ice Nucleation and Heavy Rainfall Over Arid Rajasthan, India

被引:0
|
作者
Desouza, Nirmala D. [1 ]
Blaise, D. [2 ]
Velmourougane, K. [2 ]
机构
[1] Visvesvarayya Natl Inst Technol, Dept Phys, Nagpur 440010, India
[2] ICAR Cent Inst Cotton Res, Dept Crop Prod, Nagpur 441108, India
来源
WATER AIR AND SOIL POLLUTION | 2023年 / 234卷 / 03期
基金
美国海洋和大气管理局;
关键词
AERONET; CALIPSO; HYSPLIT; Northwest India; Soot; Triticum aestivum; OPTICAL DEPTH; FAST PYROLYSIS; SATELLITE DATA; PRECIPITATION; CLOUD; BIOMASS; OZONE; DUST; AGRICULTURE; CARBON;
D O I
10.1007/s11270-023-06213-y
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In the Indo-Gangetic Plains, extensive crop residue burning (CRB) of wheat stubble is done during the month of May. Soot emitted following CRB, a serious environmental pollutant, affects cloud properties. Though important, it is poorly understood as an ice nucleating particle. During the summer season, on 13 May 2020, an unusually heavy rainfall event occurred over Rajasthan, India, which was studied using ground- and satellite-data. The sun photometer observations of the AERONET station on 12 May 2020 yielded an absorption angstrom ngstorm exponent value of 1.01. This value corresponds to black carbon (BC) and indicates its dominance as a fine aerosol associated with CRB. The HYSPLIT model indicated a downwind trajectory towards Rajasthan from Haryana and Punjab (source of CRB). Atmospheric ageing and oxygenation of BC probably increased the number of hydrophilic surface sites. Thus, soot comprising BC particles got activated into cloud droplets through the heterogeneous nucleation of water vapour. As a result, the prevailing sub-saturation condition with 80% RH led to the wetting of BC particles through the nucleation of water vapour and increased ice concentration in the cloud anvils in the late night of 12 May 2020 and precipitated on 13 May 2020 (up to 58.2 mm). AERONET data highlights that the region had an abundance of BC produced from CRB. Apart from its water affinity, other particle characteristics such as porosity and polarity also augmented ice nucleation.
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