Bubble Engineering on Micro-/Nanostructured Electrodes for Water Splitting

被引：72

作者：

Li, Mengxuan ^{[1
]}

Xie, Pengpeng ^{[1
]}

Yu, Linfeng ^{[1
]}

Luo, Liang ^{[1
]}

Sun, Xiaoming ^{[1
]}

机构：

[1] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China

来源：

ACS NANO | 2023年 / 17卷 / 23期

基金：

中国国家自然科学基金; 北京市自然科学基金;

关键词：

water splitting; micro-/nanostructured electrode; wettability; bubble engineering; mass transfer; bubble kinetics; localized electric field; directional transportation; HYDROGEN EVOLUTION; OXYGEN EVOLUTION; GAS EVOLUTION; PERFORMANCE; GROWTH; REDUCTION; DYNAMICS; ELECTROCATALYSTS; ELECTROLYZERS; NUCLEATION;

D O I：

10.1021/acsnano.3c08831

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Bubble behaviors play crucial roles in mass transfer and energy efficiency in gas evolution reactions. Combining multiscale structures and surface chemical compositions, micro-/nanostructured electrodes have drawn increasing attention. With the aim to identify the exciting opportunities and rationalize the electrode designs, in this review, we present our current comprehension of bubble engineering on micro-/nanostructured electrodes, focusing on water splitting. We first provide a brief introduction of gas wettability on micro-/nanostructured electrodes. Then we discuss the advantages of micro-/nanostructured electrodes for mass transfer (detailing the lowered overpotential, promoted supply of electrolyte, and faster bubble growth kinetics), localized electric field intensity, and electrode stability. Following that, we outline strategies for promoting bubble detachment and directional transportation. Finally, we offer our perspectives on this emerging field for future research directions.

引用

页码：23299 / 23316

页数：18

共 50 条

[1] Progress of carbon-based micro-/nanostructured hollow electrocatalysts for water splitting
Tian T.
Li N.
Yu L.
Huagong Xuebao/CIESC Journal, 2020, 71 (06): : 2466 - 2480
[2] Review: Micro- and nanostructured surface engineering for biomedical applications
Emma Luong-Van
Isabel Rodriguez
Hong Yee Low
Noha Elmouelhi
Bruce Lowenhaupt
Sriram Natarajan
Chee Tiong Lim
Rita Prajapati
Murty Vyakarnam
Kevin Cooper
Journal of Materials Research, 2013, 28 : 165 - 174
[3] Engineering of Micro- and Nanostructured Surfaces with Anisotropic Geometries and Properties
Tawfick, Sameh
De Volder, Michael
Copic, Davor
Park, Sei Jin
Oliver, C. Ryan
Polsen, Erik S.
Roberts, Megan J.
Hart, A. John
ADVANCED MATERIALS, 2012, 24 (13) : 1628 - 1674
[4] Review: Micro- and nanostructured surface engineering for biomedical applications
Luong-Van, Emma
Rodriguez, Isabel
Low, Hong Yee
Elmouelhi, Noha
Lowenhaupt, Bruce
Natarajan, Sriram
Lim, Chee Tiong
Prajapati, Rita
Vyakarnam, Murty
Cooper, Kevin
JOURNAL OF MATERIALS RESEARCH, 2013, 28 (02) : 165 - 174
[5] Nanostructured iron oxide electrodes for the water splitting reaction
Koster, Karl
Bradley, Liam
Kharel, Priti
Dawood, Farah
ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2018, 255
[6] Micro- and nanostructured optics
Wittig, LC
Kley, EB
Tünnermann, A
GLASS SCIENCE AND TECHNOLOGY, 2003, 76 : 41 - 46
[7] Micro- and nanostructured hydroxyapatitecollagen microcarriers for bone tissue-engineering applications
Perez, R. A.
Altankov, G.
Jorge-Herrero, E.
Ginebra, M. P.
JOURNAL OF TISSUE ENGINEERING AND REGENERATIVE MEDICINE, 2013, 7 (05) : 353 - 361
[8] Micro-/Nanostructured Mechanical Metamaterials
Lee, Jae-Hwang
Singer, Jonathan P.
Thomas, Edwin L.
ADVANCED MATERIALS, 2012, 24 (36) : 4782 - 4810
[9] Micro- and Nanostructures of Photoelectrodes for Solar-Driven Water Splitting
Zhang, Peng
Gao, Lian
Song, Xuefeng
Sun, Jing
ADVANCED MATERIALS, 2015, 27 (03) : 562 - 568
[10] Micro- and nanostructured optical fibres
Bartelt, Hartmut
PASSIVE COMPONENTS AND FIBER-BASED DEVICES III, PTS 1 AND 2, 2006, 6351

← 1 2 3 4 5 →