Advances in direct production of value-added chemicals via syngas conversion

被引:0
|
作者
Yunlei An [1 ,2 ]
Tiejun Lin [2 ]
Fei Yu [2 ,3 ]
Yanzhang Yang [2 ,3 ]
Liangshu Zhong [2 ]
Minghong Wu [1 ]
Yuhan Sun [2 ,4 ]
机构
[1] School of Environmental and Chemical Engineering, Shanghai University
[2] CAS Key Laboratory of Low-Carbon Conversion Science and Engineering, Shanghai Advanced Research Institute,Chinese Academy of Sciences
[3] University of the Chinese Academy of Sciences
[4] School of Physical Science and Technology, ShanghaiTech University
基金
中国国家自然科学基金;
关键词
green carbon science; syngas conversion; Fischer-Tropsh; Fischer-Tropsh to olefins; higher alcohol synthesis;
D O I
暂无
中图分类号
TQ072 [化工产品];
学科分类号
0817 ;
摘要
Syngas conversion to fuels and chemicals is one of the most challenging subjects in the field of C1 chemistry. It is considered as an attractive alternative non-petroleum-based production route. The direct synthesis of olefins and alcohols as high value-added chemicals from syngas has drawn particular attention due to its process simplicity, low energy consumption and clean utilization of carbon resource, which conforms to the principles of green carbon science. This review describes the recent advances for the direct production of lower olefins and higher alcohols via syngas conversion. Recent progress in the development of new catalyst systems for enhanced catalytic performance is highlighted. We also give recommendations regarding major challenges for further research in syngas conversion to various chemicals.
引用
收藏
页码:887 / 903
页数:17
相关论文
共 50 条
  • [1] Advances in direct production of value-added chemicals via syngas conversion
    An, Yunlei
    Lin, Tiejun
    Yu, Fei
    Yang, Yanzhang
    Zhong, Liangshu
    Wu, Minghong
    Sun, Yuhan
    [J]. SCIENCE CHINA-CHEMISTRY, 2017, 60 (07) : 887 - 903
  • [2] Advances in direct production of value-added chemicals via syngas conversion
    Yunlei An
    Tiejun Lin
    Fei Yu
    Yanzhang Yang
    Liangshu Zhong
    Minghong Wu
    Yuhan Sun
    [J]. Science China(Chemistry)., 2017, 60 (07) - 903
  • [3] Advances in direct production of value-added chemicals via syngas conversion
    Yunlei An
    Tiejun Lin
    Fei Yu
    Yanzhang Yang
    Liangshu Zhong
    Minghong Wu
    Yuhan Sun
    [J]. Science China Chemistry, 2017, 60 : 887 - 903
  • [4] Direct photocatalytic conversion of methane to value-added chemicals
    Song, Hui
    Ye, Jinhua
    [J]. TRENDS IN CHEMISTRY, 2022, 4 (12): : 1094 - 1105
  • [5] Cobalt Carbide Nanocatalysts for Efficient Syngas Conversion to Value-Added Chemicals with High Selectivity
    Lin, Tiejun
    Yu, Fei
    An, Yunlei
    Qin, Tingting
    Li, Liusha
    Gong, Kun
    Zhong, Liangshu
    Sun, Yuhan
    [J]. ACCOUNTS OF CHEMICAL RESEARCH, 2021, 54 (08) : 1961 - 1971
  • [6] Recent Advances in Direct Synthesis of Value-Added Aromatic Chemicals from Syngas by Cascade Reactions over Bifunctional Catalysts
    Kasipandi, Saravanan
    Bae, Jong Wook
    [J]. ADVANCED MATERIALS, 2019, 31 (34)
  • [7] Recent advances in artificial enzyme cascades for the production of value-added chemicals
    Wang, Zilong
    Sekar, Balaji Sundara
    Li, Zhi
    [J]. BIORESOURCE TECHNOLOGY, 2021, 323
  • [8] Catalytic Conversion of Glycerol into Hydrogen and Value-Added Chemicals: Recent Research Advances
    Hu, Yulin
    He, Quan
    Xu, Chunbao
    [J]. CATALYSTS, 2021, 11 (12)
  • [9] Advances in the solar-energy driven conversion of methanol to value-added chemicals
    Feng, Jun
    Xu, Sha
    Du, Hao
    Gong, Qiaobin
    Xie, Shunji
    Deng, Weiping
    Zhang, Qinghong
    Wang, Ye
    [J]. MOLECULAR CATALYSIS, 2022, 530
  • [10] Catalytic direct conversion of ethane to value-added chemicals under microwave irradiation
    Robinson, Brandon
    Caiola, Ashley
    Bai, Xinwei
    Abdelsayed, Victor
    Shekhawat, Dushyant
    Hu, Jianli
    [J]. CATALYSIS TODAY, 2020, 356 : 3 - 10