Interference of dissociating wave packets in the I2 molecule driven by femtosecond laser pulses

被引:0
|
作者
韩永昌 [1 ]
胡文辉 [1 ]
于杰 [1 ]
丛书林 [1 ]
机构
[1] Department of Physics,Dalian University of Technology
基金
中国国家自然科学基金;
关键词
photodissociation; interference of wave packets; I2; molecule;
D O I
暂无
中图分类号
O561 [分子物理学];
学科分类号
070203 ; 1406 ;
摘要
The interference between two dissociating wave packets of the I2 molecule driven by femtosecond laser pulses is theoretically studied by using the time-dependent quantum wave packet method.Both the internuclear distanceand velocity-dependent density functions are calculated and discussed.It is demonstrated that the interference pattern is determined by the phase difference and the delay time between two pump pulses.With two identical pulses with a delay time of 305 fs and a FWHM of 20 fs,more interference fringes can be observed,while with two pump pulses with a delay time of 80 fs and a FWHM of 20 fs,only a few interference fringes can be observed.
引用
收藏
页码:4834 / 4839
页数:6
相关论文
共 50 条
  • [1] Interference of dissociating wave packets in the I2 molecule driven by femtosecond laser pulses
    Han Yong-Chang
    Hu Wen-Hui
    Yu Jie
    Cong Shu-Lin
    CHINESE PHYSICS B, 2009, 18 (11) : 4834 - 4839
  • [2] Controlling the spreading of wave packets of a dissociating molecule
    Tiwari, Ashwani Kumar
    Moller, Klaus B.
    Henriksen, Niels E.
    CHEMICAL PHYSICS LETTERS, 2007, 450 (1-3) : 6 - 11
  • [3] Control and imaging of interfering wave packets in dissociating I2 molecules -: art. no. 033404
    Petersen, C
    Péronne, E
    Thogersen, J
    Stapelfeldt, H
    Machholm, M
    PHYSICAL REVIEW A, 2004, 70 (03): : 033404 - 1
  • [4] Manipulating molecular rotational wave packets with strong femtosecond laser pulses
    Gao, Yunan
    Wu, Chengyin
    Xu, Nan
    Zeng, Guiping
    Jiang, Hongbing
    Yang, Hong
    Gong, Qihuang
    PHYSICAL REVIEW A, 2008, 77 (04):
  • [5] Imaging and control of interfering wave packets in a dissociating molecule
    Skovsen, E
    Machholm, M
    Ejdrup, T
    Thogersen, J
    Stapelfeldt, H
    PHYSICAL REVIEW LETTERS, 2002, 89 (13) : 133004 - 133004
  • [6] Single-collision caging of dissociating I2:: wave packet calculations and simulation of femtosecond spectra
    Meier, C
    Engel, V
    Beswick, JA
    CHEMICAL PHYSICS LETTERS, 1998, 287 (5-6) : 487 - 495
  • [7] Interference of electron wave packets in photoionization of H2+ by attosecond ultraviolet laser pulses
    Yu, Hua-Ming
    Yuan, Kai-Jun
    JOURNAL OF MODERN OPTICS, 2017, 64 (14) : 1411 - 1418
  • [8] Interference of electron wave packets in atomic ionization by subcycle sculpted laser pulses
    Arbo, Diego G.
    Nagele, Stefan
    Tong, Xiao-Min
    Xie, Xinhua
    Kitzler, Markus
    Burgdoerfer, Joachim
    PHYSICAL REVIEW A, 2014, 89 (04):
  • [9] CONTROLLING WAVE PACKET INTERFERENCE OF DISSOCIATING MOLECULES BY SHAPING LASER PULSES IN FREQUENCY DOMAIN
    Han, Yong-Chang
    Yuan, Kai-Jun
    Cong, Shu-Lin
    JOURNAL OF THEORETICAL & COMPUTATIONAL CHEMISTRY, 2008, 7 (06): : 1159 - 1169
  • [10] Vibrational wavepacket motion in I2 excited with femtosecond laser pulses in the 200 nm wavelength region
    Farmanara, P
    Ritze, HH
    Stert, V
    Radloff, W
    CHEMICAL PHYSICS LETTERS, 1999, 307 (1-2) : 1 - 7