A Z-scheme heterojunction of ZnO/CDots/C3N4 for strengthened photoresponsive bacteria-killing and acceleration of wound healing

被引:5
|
作者
Yiming Xiang [1 ,2 ,3 ]
Qilin Zhou [1 ]
Zhaoyang Li [2 ]
Zhenduo Cui [2 ]
Xiangmei Liu [1 ]
Yanqin Liang [2 ]
Shengli Zhu [2 ]
Yufeng Zheng [4 ]
Kelvin Wai Kwok Yeung [3 ]
Shuilin Wu [1 ,2 ]
机构
[1] Hubei Key Laboratory of Polymer Materials, Ministry-of-Education Key Laboratory for the Green Preparation and Application of Functional Materials,School of Materials Science & Engineering, Hubei University
[2] The Key Laboratory of Advanced Ceramics and Machining Technology by the Ministry of Education of China, School of Materials Science & Engineering,Tianjin University
[3] Department of Orthopaedics & Traumatology, Li Ka Shing Faculty of Medicine, The University of Hong Kong
[4] State Key Laboratory for Turbulence and Complex System and Department of Materials Science and Engineering, College of Engineering, Peking University
基金
中国国家自然科学基金; 国家重点研发计划;
关键词
D O I
暂无
中图分类号
R318.08 [生物材料学];
学科分类号
0805 ; 080501 ; 080502 ;
摘要
The abuse of antibiotics is leading to the emergence of resistant bacteria. In this work, a drug-free composite of ZnO/CDots/g-CNwith Z-scheme heterojunction was developed, which was employed to kill bacteria effectively within a very short time under the irradiation of visible light due to the enhanced photocatalytic and photothermal effects. In this system, the CDots acted as a bridge between g-CNand ZnO, effectively inhibiting the recombination of photo-generated electrons with holes and consequently enhancing the photocatalytic properties. In addition, CDots endowed the system with excellent photothermal effects. As a result, the antibacterial efficacy of ZnO/CDots/g-CNcomposite against S. aureus and E. coli reached up to 99.97 % and 99.99 % respectively, after 15 min of visible light irradiation, due to the synergistic action of photo-inspired radical oxygen species and hyperthermia. The Zn ions released from the composite promoted the growth of fibroblasts, which accelerated the wound healing process.
引用
收藏
页码:1 / 11
页数:11
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