Quantification of Fugitive Carbon Emissions from Uncontrolled Combustion in Coal Fire Area: the Sandaoba Coalfield, Xinjiang, China

被引:0
|
作者
Deng, Jinchang [1 ,2 ]
Shi, Bobo [4 ]
Cullen, Jose L. Torero [5 ]
Xue, Yong [2 ]
Zhou, Fubao [3 ]
机构
[1] Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Atmospher Environm & Equipm, Sch Environm Sci & Engn, Jiangsu Key Lab Atmospher Environm Monitoring & Po, Nanjing 210044, Peoples R China
[2] Nanjing Univ Informat Sci & Technol, Sch Emergency Management, Nanjing 210044, Peoples R China
[3] China Acad Safety Sci & Technol, Beijing 100012, Peoples R China
[4] China Univ Min & Technol, Sch Safety Engn, Xuzhou 221116, Peoples R China
[5] UCL, Dept Civil Environm & Geomat Engn, London WC1E6BT, England
基金
中国博士后科学基金; 中国国家自然科学基金;
关键词
Coal fires; Emission flux model; Field measurements; Geostatistical analysis; CO; 2; estimation; GREENHOUSE-GAS EMISSIONS; GASEOUS EMISSIONS; KENTUCKY; CO2;
D O I
10.1016/j.envres.2025.120923
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Spontaneous coal fires are a significant source of greenhouse gas emissions, contributing to global warming. However, the lack of reliable estimation methods and research has obscured the full environmental impact of these emissions. This paper presents a novel quantification method for fugitive carbon emissions from spontaneous coal combustion. A combination of field measurements, laboratory tests, and geostatistical analysis led to the development of the Carbon Emission Flux (CEF) model, which was applied to the Sandaoba coalfield fire areas. The study quantitatively estimates the average CO2 emission fluxes from borehole, fissure, and soil sources: 517 g/m2 center dot s, 61.5 g/m2 center dot s and 5.33 mg/m2 center dot s, respectively. Borehole fluxes exhibit the highest intensity, while fissures contribute the most carbon emissions. Both temperature and gas velocity significantly and positively influence the CO2 concentration in borehole and fissure emissions. Surface fissure density, measured across different fire areas, averages 1.039 x 10-3 per unit area. Using chamber flux measurement and Kriging geostatistical interpolation, the net soil-diffuse flux was determined to be 2.406 mg/m2 center dot s after background removal. Methane emissions are also considered, with a correction factor of 1.004%. The total annual fugitive carbon emissions from the Sandaoba coalfield fire are estimated at (6.53 +/- 1.86) x 105 tons/yr (COQ equivalent), with a robust uncertainty of 28.6%. The study further highlights the significant carbon reduction achieved through local fire suppression efforts, applicable across all emission sources.
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页数:13
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