Topologically Engineered High-Q Quasi-BIC Metasurfaces for Enhanced Near-Infrared Emission in PbS Quantum Dots

被引:0
|
作者
Guo, Jiaoyang [1 ,2 ]
Jin, Rong [1 ,2 ]
Fu, Zhenchu [1 ,2 ]
Zhang, Yukang [1 ,2 ]
Yu, Feilong [1 ,2 ]
Chen, Jin [1 ,2 ]
Wang, Xingjun [5 ,6 ]
Huang, Lujun [3 ]
Zhou, Chaobiao [7 ]
Chen, Xiaoshuang [1 ,2 ,4 ]
Lu, Wei [1 ,2 ,4 ]
Li, Guanhai [1 ,2 ,4 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Tech Phys, State Key Lab Infrared Phys, Shanghai 200083, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] East China Normal Univ, Sch Phys & Elect Sci, Shanghai 200241, Peoples R China
[4] Shanghai Res Ctr Quantum Sci, Shanghai 201315, Peoples R China
[5] Univ Shanghai Sci & Technol, Coll Sci, Shanghai 200093, Peoples R China
[6] Univ Shanghai Sci & Technol, Terahertz Technol Innovat Res Inst, Terahertz Spectrum & Imaging Technol Cooperat Inno, Shanghai Key Lab Modern Opt Syst, Shanghai 200093, Peoples R China
[7] Guizhou Minzu Univ, Sch Phys & Mechatron Engn, Guiyang 550025, Peoples R China
基金
中国国家自然科学基金;
关键词
quasi-bound state in the continuum; photoluminescenceenhancement; PbS quantum dots; FLUORESCENCE; FANO;
D O I
10.1021/acs.nanolett.4c05710
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Enhancing photoluminescence (PL) efficiency in colloidal quantum dots is pivotal for next-generation near-infrared photodetectors, imaging systems, and photonic devices. Conventional methods, especially metal-based plasmonic structures, suffer from large optical losses, which limits their practical use. Here, we introduce a quasi-bound state in the continuum (quasi-BIC) metasurface on a silicon-on-insulator platform, tailored to provide high-quality factor resonances with minimized losses. Utilizing topological charge engineering and controlled in-plane asymmetry in silicon cylinder arrays, we developed a robust quasi-BIC capable of maintaining a high Q factor across a broad angular range, achieving an experimental Q factor of 3031 at normal incidence. This approach significantly enhances near-field interactions, achieving a <= 110-fold increase in PL for PbS quantum dots at 33 K and a 41-fold enhancement at room temperature. Our findings offer a scalable, cost-effective solution for enhancing light emission in advanced optoelectronic applications.
引用
收藏
页码:2357 / 2365
页数:9
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