Reentrant multiple-<bold>q</bold> magnetic order and a "spin meta-cholesteric" phase in Sr3Fe2O7

被引:0
|
作者
Andriushin, N. D. [1 ]
Muller, J. [2 ]
Pavlovskii, N. S. [1 ]
Grumbach, J. [1 ]
Granovsky, S. [1 ]
Tymoshenko, Y. V. [1 ]
Zaharko, O. [3 ]
Ivanov, A. [4 ]
Ollivier, J. [4 ]
Doerr, M. [1 ]
Keimer, B. [5 ]
Mostovoy, M. [2 ]
Inosov, D. S. [1 ,6 ]
Peets, D. C. [1 ,5 ]
机构
[1] Tech Univ Dresden, Inst Festkorper & Materialphys, Dresden, Germany
[2] Univ Groningen, Zernike Inst Adv Mat, Groningen, Netherlands
[3] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, Villigen, Switzerland
[4] Inst Laue Langevin, Grenoble, France
[5] Max Planck Inst Festkorperforsch, Stuttgart, Germany
[6] Tech Univ Dresden, Wurzburg Dresden Cluster Excellence Complex & Topo, Dresden, Germany
关键词
CRYSTALS; STATE;
D O I
10.1038/s41535-024-00698-4
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Topologically nontrivial magnetic structures such as skyrmion lattices are well known in materials lacking lattice inversion symmetry, where antisymmetric exchange interactions are allowed. Only recently, topological multi-q magnetic textures that spontaneously break the chiral symmetry, for example, three-dimensional hedgehog lattices, were discovered in centrosymmetric compounds, where they are instead driven by frustrated interactions. Here we show that the bilayer perovskite Sr3Fe2O7, previously believed to adopt a simple single-q spin-helical order, hosts two distinct types of multi-q spin textures. Its ground state represents a novel multi-q spin texture with unequally intense spin modulations at the two ordering vectors. This is followed in temperature by a new "spin meta-cholesteric" phase, in which the chiral symmetry is spontaneously broken along one of the crystal directions, but the weaker orthogonal modulation melts, giving rise to intense short-range dynamical fluctuations. Shortly before the transition to the paramagnetic state, vortex-crystal order spanned by two equivalent q vectors emerges. This renders Sr3Fe2O7 an ideal material to study transitions among multiple-q spin textures in a centrosymmetric host.
引用
收藏
页数:6
相关论文
共 11 条
  • [1] Rich magnetic phase diagram of putative helimagnet Sr3Fe2O7
    Andriushin, Nikita D.
    Grumbach, Justus
    Kim, Jung-Hwa
    Reehuis, Manfred
    Tymoshenko, Yuliia, V
    Onykiienko, Yevhen A.
    Jain, Anil
    Macfarlane, W. Andrew
    Maljuk, Andrey
    Granovsky, Sergey
    Hoser, Andreas
    Pomjakushin, Vladimir
    Ollivier, Jacques
    Doerr, Mathias
    Keimer, Bernhard
    Inosov, Dmytro S.
    Peets, Darren C.
    PHYSICAL REVIEW B, 2023, 108 (17)
  • [2] Charge disproportionation and antiferromagnetic order of Sr3Fe2O7
    Kuzushita, K
    Morimoto, S
    Nasu, S
    Nakamura, S
    JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2000, 69 (09) : 2767 - 2770
  • [3] Magnetic solid phase extraction of copper from aquatic samples by Fe<bold>3</bold>O<bold>4</bold>/SiO<bold>2</bold> nanoparticles followed by atomic absorption spectrometric determination
    Khoshhesab, Zahra Monsef
    Mirzaie, Afsaneh
    SEPARATION SCIENCE AND TECHNOLOGY, 2016, 51 (10) : 1654 - 1663
  • [4] Thermodynamic investigation of the Ruddlesden-Popper phase Sr3Fe2O7
    Knyazev, A. V.
    Alekseeva, Yu. V.
    Smirnova, N. N.
    Krasheninnikova, O. V.
    Markin, A. V.
    Syrov, E. V.
    Elipasheva, E. V.
    Smirnova, L. V.
    JOURNAL OF CHEMICAL THERMODYNAMICS, 2020, 143 (143):
  • [5] Magnetic phase diagram of Sr3Fe2O7-δ
    Peets, D. C.
    Kim, J. -H.
    Dosanjh, P.
    Reehuis, M.
    Maljuk, A.
    Aliouane, N.
    Ulrich, C.
    Keimer, B.
    PHYSICAL REVIEW B, 2013, 87 (21):
  • [6] STRUCTURE AND MAGNETIC-PROPERTIES OF SR2FEO4 AND SR3FE2O7 STUDIED BY POWDER NEUTRON-DIFFRACTION AND MOSSBAUER-SPECTROSCOPY
    DANN, SE
    WELLER, MT
    CURRIE, DB
    THOMAS, MF
    ALRAWWAS, AD
    JOURNAL OF MATERIALS CHEMISTRY, 1993, 3 (12) : 1231 - 1237
  • [7] Nonthermal breaking of magnetic order via photogenerated spin defects in the spin-orbit coupled insulator Sr3Ir2O7
    Pastor, Ernest
    Moreno-Mencia, David
    Monti, Maurizio
    Johnson, Allan S.
    Fleischmann, Nina
    Wang, Cuixiang
    Shi, Youguo
    Liu, Xuerong
    Mazzone, Daniel G.
    Dean, Mark P. M.
    Wall, Simon
    PHYSICAL REVIEW B, 2022, 105 (06)
  • [8] Tuning of structural phase, magnetic spin order and electrical conductivity in mechanical alloyed material of α-Fe2O3 and α-Cr2O3 oxides
    Bhowmik, R. N.
    Siva, K. Venkata
    Reddy, V. R.
    Sinha, A. K.
    JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2020, 514
  • [9] Multiple magnetic phase transitions in single-crystal (Sr1-xCax)3Ru2O7 for 0 o x o 1.0
    Cao, G.
    McCall, S. C.
    Crow, J. E.
    Guertin, R. P.
    Physical Review B: Condensed Matter, 56 (09):
  • [10] Multiple magnetic phase transitions in single-crystal (Sr1-xCax)(3)Ru2O7 for 0<=X<=1.0
    Cao, G
    McCall, SC
    Crow, JE
    Guertin, RP
    PHYSICAL REVIEW B, 1997, 56 (09): : 5387 - 5394