The application of high-frequency/high-field electron paramagnetic resonance in the research on spin qudits

被引:0
|
作者
Yuan J. [1 ,2 ]
Fu P. [3 ]
Gao S. [3 ]
Jiang S. [2 ]
Zhou S. [1 ]
机构
[1] Institute for Quantum Information Science and technology, College of Science, National University of Defense Technology, Changsha
[2] Spin-X Institute, South China University of Technology, Guangzhou
[3] College of Chemistry and Molecular Engineering, Peking University, Beijing
关键词
electric spin resonance; electron spin; molecular spin qudits; quantum coherent manipulation;
D O I
10.19650/j.cnki.cjsi.J2312027
中图分类号
学科分类号
摘要
Electron spin resonance (EPR) is a powerful technique to study the electron structure and dynamics of many materials with unpaired electrons (paramagnetic materials). Nowadays, EPR has been widely applied in chemistry, material, radiation detection, biology, and quantum information processing. Compared with the X-Band EPR, the high frequency/ field EPR (HF-EPR) has the advantages of resolution, sensitivity, and initialization. This article is a concise introduction to the history, basic theory, instrumentation, and characteristics of the HF-EPR, and the emphasis on the application of HF-EPR in the research on spin qudits. The progress and future prospects of this analysis technique are also outlined. The HF-EPR could be used as a tool to implement the coherent manipulation of spin qudits, further paving the way toward quantum logic gate operation and quantum algorithm. © 2024 Science Press. All rights reserved.
引用
收藏
页码:144 / 156
页数:12
相关论文
共 57 条
  • [1] WEIL J A, BOLTON J R., Electron Paramagnetic Resonance: Elementary Theory and Practical Applications, (2007)
  • [2] ZHOU S, YUAN J, WANG Z Y, Et al., Implementation of quantum level addressability and geometric phase manipulation in aligned endohedral fullerene qudits, Angewandte Chemie, (2022)
  • [3] FU P X, ZHOU S, LIU Z, Et al., Multiprocessing quantum computing through hyperfine couplings in endohedral fullerene derivatives [ J ], Angewandte Chemie, (2022)
  • [4] WANG Y X, LIU Z, FANG Y H, Et al., Coherent manipulation and quantum phase interference in a fullerene-based electron triplet molecular qutrit, NPJ Quantum Information, 7, 1, (2021)
  • [5] LIU Z, WANG Y X, FANG Y H, Et al., Electric field manipulation enhanced by strong spin-orbit coupling: promoting rare-earth ions as qubits, National Science Review, 7, 10, pp. 1557-1563, (2020)
  • [6] FANG Y H, LIU Z, ZHOU S, Et al., Spin-electric coupling with anisotropy-induced vanishment and enhancement in molecular ferroelectrics, Journal of the American Chemical Society, 144, 19, pp. 8605-8612, (2022)
  • [7] WANG Y, CHEN Y, BUI H T, Et al., An atomic-scale multi-qubit platform, Science, 382, 6666, pp. 87-92, (2023)
  • [8] SELLIES L, SPACHTHOLZ R, BLEHER S, Et al., Single-molecule electron spin resonance by means of atomic force microscopy [ J ], Nature, 624, 7990, pp. 64-68, (2023)
  • [9] WANG Z, BALEMBOIS L, RANCIC M, Et al., Single-electron spin resonance detection by microwave photon counting, Nature, 619, 7969, pp. 276-281, (2023)
  • [10] SMITH G M, CRUICKSHANK P A S, BOLTON D R, Et al., High-field pulse EPR instrumentation, Electron Paramagnetic Resonance, (2008)