Review: Two-dimensional nanostructured pristine graphene and heteroatom-doped graphene-based materials for energy conversion and storage devices

被引：0
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作者：
Chowdury, Md Shahjahan Kabir [1 ]
Park, Ye Ji [1 ]
Park, Sung Bum [2 ]
Park, Yong-il [1 ]
机构：
[1] School of Materials Science and Engineering, Kumoh National Institute of Technology, 61 Daehak-ro, Gyeongbuk, Gumi,39177, Korea, Republic of
[2] Department of Automotive Materials and Components Engineering, Dongguk University WISE Campus, Gyeongju,38066, Korea, Republic of
来源：
Sustainable Materials and Technologies | 2024年 / 42卷
关键词：
With the goal of achieving net zero carbon emissions and the growing scarcity of fossil fuels; significant efforts have been devoted to the development of high-efficiency; low-cost; environmentally friendly; and alternative energy conversion and storage devices. Pristine graphene; consisting of single-atom-thick carbon nanosheets arranged in an sp2 hybridized honeycomb lattice; has emerged as a primary building-block material; including a large surface area; mechanical strength; chemical inertness; and superior electric and thermal properties. Since pristine graphene has a band gap of zero; which significantly limits its applications; modifying graphene by incorporating a heteroatom is a highly effective method to enhance its properties. This approach enhances the suitability and potential of heteroatom-doped graphene as an electrode material in energy conversion and storage devices. This review comprehensively describes the current synthesis advancements in pristine graphene; and heteroatom-doped graphene-based electrocatalysts and/or electrode materials for two types of energy conversion: fuel cells; and water splitting; as well as three frontier energy storage devices; namely supercapacitors and lithium-based various types of batteries. To this end; an exploration of the future prospects; opportunities; and challenges pertaining to the application of graphene and its heteroatom-doped graphene in energy conversion and storage devices is anticipated. This comprehensive review article aims to pave the way for novel advancements and practical utilization of heteroatom-doped graphene-based materials in various domains. © 2024;
D O I：
10.1016/j.susmat.2024.e01124
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