Silicon carbon-supported copper oxide catalysts for the selective catalytic reduction of NOx with NH3 at low temperature

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作者
Bai, Shu-Li [1 ]
Zhang, Xiao-Yu [1 ]
Xue, Yao-Jia [1 ]
Li, Huan-Ying [1 ]
Jia, Jian-Bo [1 ]
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[1] School of Biotechnology and Health Sciences, Wuyi University, Jiangmen,529020, China
关键词
Silicon carbide supported copper oxide (CuO/SiC) catalysts were prepared by wet impregnation method and characterized by scanning electron microscope (SEM); X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS); their catalytic performance in the selective catalytic reduction of NOx with NH3 at low temperature was investigated with a mimic flue gas. The results indicate that the catalytic performance of CuO/SiC in the selective catalytic reduction NO with NH3 is related to the loading of copper oxide and reaction temperature. The CuO/SiC catalyst with a CuO loading of 5% exhibits high activity at low temperature; where SO2 shows slightly inhibition upon the NO reduction activity; the NO reduction reaction over CuO/SiC may take place between the adsorbed ammonia and the gaseous or weakly adsorbed NO. Such CuO/SiC catalysts may provide a new choice for the practical removal of NOx in industry. © 2020; Science Press. All right reserved;
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页码:723 / 727
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