Life cycle assessment of hydrogenotrophic denitrification in membrane aerated biofilm reactors for sustainable wastewater treatment
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作者:
Li, Rui
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机构:
Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Shandong Energy Inst, Qingdao 266101, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Li, Rui
[1
,2
,3
]
Lu, Ming-yi
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机构:
Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Shandong Energy Inst, Qingdao 266101, Peoples R ChinaChinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Lu, Ming-yi
[1
,2
]
Guo, Rong-bo
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机构:
Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Shandong Energy Inst, Qingdao 266101, Peoples R ChinaChinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Guo, Rong-bo
[1
,2
]
Duan, Haoran
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机构:
Univ New South Wales, Sch Civil & Environm Engn, Sydney, NSW 2052, AustraliaChinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Duan, Haoran
[4
]
Ni, Bing-jie
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Univ New South Wales, Sch Civil & Environm Engn, Sydney, NSW 2052, AustraliaChinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Ni, Bing-jie
[4
]
Fu, Shan-fei
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机构:
Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Shandong Energy Inst, Qingdao 266101, Peoples R ChinaChinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
Fu, Shan-fei
[1
,2
]
机构:
[1] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Shandong Engn Res Ctr Biogas, Qingdao New Energy Shandong Lab, Qingdao 266101, Peoples R China
[2] Shandong Energy Inst, Qingdao 266101, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[4] Univ New South Wales, Sch Civil & Environm Engn, Sydney, NSW 2052, Australia
Membrane aerated biofilm reactors;
Hydrogenotrophic denitrification;
Life cycle assessment;
D O I:
10.1016/j.watres.2024.122529
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
The conventional anaerobic-anoxic-oxic (AAO) process for wastewater treatment is associated with high energy consumption and pollutant emissions due to its reliance on heterotrophic denitrification. In contrast, membrane aerated biofilm reactors (MABR) coupled with hydrogenotrophic denitrification (H-2-MABR) offers a more promising alternative. This study conducts a life cycle assessment (LCA) to evaluate the environmental and economic benefits of H-2-MABR compared to traditional AAO processes. Results indicate that even with a limited reactor life, the application of MABR in actual wastewater treatment plants can yield over 30 % reduction in environmental and economic impacts. Using CO2 from biogas as a carbon source significantly reduces carbon emissions during the anaerobic stage, while the efficient nitrogen removal minimizes the need for wastewater recirculation and electricity consumption. The H-2-driven denitrification process also avoids emissions and secondary pollution risks associated with organic electron donors. Furthermore, coupling H-2-MABR with renewable energy source and Power-to-Gas technology further enhances sustainability by ensuring a stable hydrogen supply. Given the significant potential of H-2-MABR for improving wastewater treatment, further research and large-scale implementation are highly encouraged.
机构:
Qatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, QatarQatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, Qatar
Dicataldo, Gennaro
Desmond, Peter
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机构:
Hamad Bin Khalifa Univ, Coll Sci & Engn, Doha, QatarQatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, Qatar
Desmond, Peter
Al-Maas, Mashael
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机构:
Qatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, QatarQatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, Qatar
Al-Maas, Mashael
Adham, Samer
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机构:
Qatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, Qatar
Qatar Univ, Ctr Adv Mat, POB 2713, Doha, QatarQatar Sci & Technol Pk, ConocoPhillips Global Water Sustainabil Ctr, POB 24750, Doha, Qatar
机构:
Tongji Univ, Shanghai Inst Pollut Control & Ecol Secur, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R ChinaTongji Univ, Shanghai Inst Pollut Control & Ecol Secur, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R China
Li, Jia
Wang, Zhiwei
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机构:
Tongji Univ, Shanghai Inst Pollut Control & Ecol Secur, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R ChinaTongji Univ, Shanghai Inst Pollut Control & Ecol Secur, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R China
Wang, Zhiwei
Wang, Yayi
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机构:
Tongji Univ, Shanghai Inst Pollut Control & Ecol Secur, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R ChinaTongji Univ, Shanghai Inst Pollut Control & Ecol Secur, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R China
机构:
Lakehead Univ, Dept Chem Engn, 955 Oliver Rd, Thunder Bay, ON P7B 5E1, CanadaLakehead Univ, Dept Chem Engn, 955 Oliver Rd, Thunder Bay, ON P7B 5E1, Canada
Zheng, M. R.
Liao, B. Q.
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Lakehead Univ, Dept Chem Engn, 955 Oliver Rd, Thunder Bay, ON P7B 5E1, CanadaLakehead Univ, Dept Chem Engn, 955 Oliver Rd, Thunder Bay, ON P7B 5E1, Canada