Effects of CO 2 /H 2 O Addition on Soot Reactions in n-Butanol Flames

被引:0
|
作者
Qiu L. [1 ]
Li Z. [1 ]
Liu Y. [1 ]
Qin L. [1 ]
Cheng X. [1 ]
机构
[1] School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan
来源
Cheng, Xiaobei (xbcheng@hust.edu.cn) | 2018年 / Chinese Society for Internal Combustion Engines卷 / 36期
关键词
Coflow diffusion flame; N-butanol; Soot mass fraction; Soot number density;
D O I
10.16236/j.cnki.nrjxb.201805058
中图分类号
学科分类号
摘要
The effects of CO 2 or water vapor addition to the air stream on the soot mass fractions(SMF)and soot number densities were numerically investigated in a laminar coflow n-butanol/air diffusion flame based on a reduced nbutanol mechanism and a fixed sectional soot model. Results show that both the SMF and number densities are reduced as CO 2 or H 2 O vapor is added. Besides, the reactions and concentration distributions of species move downstream with the addition of CO 2 . The decrease of soot number density is caused by the drop of temperature and mole fraction of pyrene(A4)that leads to a decrease of inception rate. While the decrease of soot mass fraction is caused by the drop of temperature, mole fraction of H and total surface area of particles that leads to a decrease of hydrogenabstraction- carbon-addition(HACA)rate. Finally, all the particles are completely oxidized, with the major oxidizing component being OH. © 2018, Editorial Office of the Transaction of CSICE. All right reserved.
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页码:447 / 454
页数:7
相关论文
共 23 条
  • [1] Myung C.L., Park S., Exhaust nanoparticle emissions from internal combustion engines: A review, International Journal of Automotive Technology, 13, 1, pp. 9-22, (2012)
  • [2] Jacobson M.Z., Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols, Nature, 409, pp. 695-697, (2001)
  • [3] Choi S., Myung C.L., Park S., Review on characterization of nano-particle emissions and PM morphology from internal combustion engines: Part 2, International Journal of Automotive Technology, 15, 2, pp. 219-227, (2014)
  • [4] Megaridis C.M., Dobbins R.A., Soot aerosol dynamics in a laminar ethylene diffusion flame, Symposium(International)on Combustion, 22, 1, pp. 353-362, (1989)
  • [5] Liu F., Guo H., Smallwood G.J., Et al., Numerical modelling of soot formation and oxidation in laminar coflow non-smoking and smoking ethylene diffusion flames, Combustion Theory and Modelling, 7, 2, pp. 301-315, (2003)
  • [6] Dogan O., The influence of n-butanol/diesel fuel blends utilization on a small diesel engine performance and emissions, Fuel, 90, 7, pp. 2467-2472, (2011)
  • [7] Guo H., Smallwood G.J., A numerical study on the influence of CO <sub>2</sub> addition on soot formation in an ethylene/air diffusion flame , Combustion Science and Technology, 180, 10-11, pp. 1695-1708, (2008)
  • [8] Liu F., Consalvi J., Fuentes A., Effects of water vapor addition to the air stream on soot formation and flame properties in a laminar coflow ethylene/air diffusion flame, Combustion and Flame, 161, 7, pp. 1724-1734, (2014)
  • [9] Eaves N.A., Zhang Q., Liu F., Et al., CoFlame: A refined and validated numerical algorithm for modeling sooting laminar coflow diffusion flames, Computer Physics Communications, 207, pp. 464-477, (2016)
  • [10] Zhang Q., Detailed modeling of soot formation/oxidation in laminar coflow diffusion flames, (2009)