Microreactor with silver-loaded metal-organic framework films for gas-phase reactions

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作者：
机构：
[1] Papurello, Rocío L.
[2] Fernández, José L.
[3] Miró, Eduardo E.
[4] Zamaro, Juan M.
来源：
Zamaro, Juan M. (zamaro@fiq.unl.edu.ar) | 1600年 / Elsevier B.V., Netherlands卷 / 313期
关键词：
Gases - Silver compounds - Carbon monoxide - Catalytic oxidation - Crystalline materials - Microchannels - Film growth - Silver - Phase interfaces;
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摘要：
Microreactors of copper foils with microchannels having zeolitic imidazolate framework-8 (ZIF-8) films were developed. The films were obtained by direct solvothermal synthesis on the microchannels; they presented micrometric thicknesses and homogeneity, and were activated with highly dispersed silver species. The MOF-based microreactors showed high activity and stability in the carbon monoxide oxidation, which is a benchmark for exothermic gas-phase reactions. The results could bring new perspectives in the development of microreactors for heterogeneous catalytic gas-phase reactions based on other MOF films as supports of active phases. © 2016 Elsevier B.V.
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