Distribution, sources and risk assessment of the PAHs in the surface sediments and water from the daye lake

被引：7
|
作者：
Zhang J.-Q. [1 ]
Hu T.-P. [1 ,2 ]
Xing X.-L. [2 ]
Zheng H. [2 ]
Zhang L. [1 ]
Zhan C.-L. [1 ]
Liu H.-X. [1 ]
Xiao W.-S. [1 ]
Qi S.-H. [2 ]
机构：
[1] School of Environmental Science and Engineering, Hubei Polytechnic University, Huangshi
[2] School of Environmental Studies, China University of Geosciences, Wuhan
来源：
Huanjing Kexue/Environmental Science | 2017年 / 38卷 / 01期
关键词：
Daye Lake; Health risk; PAHs; Source apportionment; Surface sediments; Water;
D O I：
10.13227/j.hjkx.201606058
中图分类号：
学科分类号：
摘要：
8 surface sediments and 8 water samples were collected from the Daye Lake in August 2015. The 16 kinds of EPA control polycyclic aromatic hydrocarbons (PAHs) were analyzed by GC-MS. The results showed that the PAHs concentrations of surface sediments and water ranged from 35.94 ng·g-1 to 2 032.73 ng·g-1 and from 27.94 ng·L-1 to 242.95 ng·L-1, with average contents of 940.61 ng·g-1 and 107.77ng·L-1, respectively. The distribution of PAHs in surface sediments indicated that the contents in the center samples were higher than those in the bank samples, but the water showed nearly the opposite tendency. The 4-5 rings high molecular weight PAHs were the main components in the surface sediments, and the 2, 4 and 5 rings PAHs were given priority in water. Compared with the other domestic and oversea lakes, the PAHs pollution of the Daye Lake was at a moderate level. Source apportionment showed that the PAHs in surface sediments and water from the Daye Lake came from the combustion source, HWM-PAHs were the dominant part of the PAHs in the sediment, reflecting the sediment PAHs pollution under the effects of mining and smelting over a long period; All monomer PAHs and total PAHs content in sediment did not exceed the ERM and FEL limiting values, showing that there was no particularly serious ecological risk caused by PAHs in the surface sediments from the Daye Lake; the incremental lifetime cancer risks assessment showed that the uptake risk of PAHs in Daye Lake water through the ingestion and dermal absorption were both in the acceptable range recommended by the USEPA, but all sites had higher risk than the acceptable risk level recommended by the Sweden environmental protection agency and Royal society. The pollution of seven carcinogenic PAHs needs prevention and control. © 2017, Science Press. All right reserved.
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页码：170 / 179
页数：9
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