Difference in PM2.5 Pollution and Transport Characteristics Between Urban and Suburban Areas

被引:1
|
作者
Qi P. [1 ]
Zhou Y. [1 ]
Cheng S.-Y. [1 ]
Bai W.-C. [1 ]
机构
[1] Key Laboratory of Beijing on Regional Air Pollution Control, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing
来源
Huanjing Kexue/Environmental Science | 2022年 / 43卷 / 11期
关键词
boundary layer height; PM[!sub]2.5[!/sub; suburbs; transport characteristics; urban areas;
D O I
10.13227/j.hjkx.202201227
中图分类号
学科分类号
摘要
Based on multi-source observation data, such as lidar ceilometer, aircraft AMDAR, and conventional sites, combined with numerical simulation (CAMx-PSAT), this study took the typical cities of the Beijing-Tianjin-Hebei region—Beijing (BJ) urban area and suburbs (Miyun) and Shijiazhuang (SJZ) urban area and suburbs (Pingshan) as the case study areas. The differences in boundary layer height between urban areas and suburbs (ΔPBLH), surface PM2.5 mass concentration (ΔSurf-PM2.5), vertical PM2.5 mass concentration (ΔVert-PM2.5), and transmission flux intensity and height distribution characteristics were analyzed. The results showed: due to factors such as anthropogenic heat sources, short-wave radiation, and thermal turbulence, the annual average planetary boundary layer height in urban areas was 8%-29% higher than that in the suburbs, and in different seasons, the monthly average planetary boundary layer height in urban areas was 2% (April in SJZ)-47% (July in BJ) higher than that in the suburbs. Due to the combined effects of anthropogenic emissions, inversions, and atmospheric turbulence, the annual averageρ(PM2.5) in urban areas between 0-1260 m was higher than that in suburbs by 0. 1 (SJZ)-29. 7 (BJ) μg·m -3 and decreased with the increase in height. The annual average total net flux intensity in urban areas was much greater than that in suburbs, with outflows in urban areas and inflows in suburbs; due to the urban low pressure and the suburban high pressure, suburban thermal circulation was formed. The annual average total net flux intensity in BJ (44.77 t·d -1) was greater than that in SJZ (34. 44 t·d -1). Affected by wind speed and PM2.5 mass concentration, between 0-1260 m, the fluxes in urban areas and suburbs and surrounding areas showed an obvious trend of increasing net flux intensity with the increase in height above the ground. Furthermore, the transmission exchange between urban areas and suburbs and surrounding areas in January and April had the most obvious impact on the environment. The intensity of the maximum net flux in the lower urban areas and the suburbs in different seasons was significantly different, and the difference between the two was 2. 23-4. 48 times; however, the height characteristic difference in the intensity of the maximum net flux was small, mainly located at 611-1 260 m. © 2022 Science Press. All rights reserved.
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页码:5018 / 5029
页数:11
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共 49 条
  • [1] Song J, Lim Y C, Ko I, Et al., Association between air pollutants and initial hospital admission for ischemic stroke in Korea from 2002 to 2013 [ J ], Journal of Stroke and Cerebrovascular Diseases, 30, 11, (2021)
  • [2] Singer B C, Zhao H R, Preble C V, Et al., Measured influence of overhead HVAC on exposure to airborne contaminants from simulated speaking in a meeting and a classroom, Indoor Air, 32, 1, (2022)
  • [3] Wang X R, Miao S G, Dou J X, Et al., Observation and analysis of the air pollution impacts on radiation balance of urban and suburb areas in Beijing, Chinese Journal of Geophysics, 59, 11, pp. 3996-4006, (2016)
  • [4] Liu Y S, Tang G Q, Huang X J, Et al., Unexpected deep mixing layer in the Sichuan basin, China, Atmospheric Research, 249, (2021)
  • [5] Yang L, He K B, Zhang Q, Et al., Vertical distributive characters of PM<sub>2.5</sub> at the ground layer in autumn and winter in Beijing, Research of Environmental Sciences, 18, 2, pp. 23-28, (2005)
  • [6] Lei L, Sun Y L, Ouyang B, Et al., Vertical distributions of primary and secondary aerosols in Urban boundary layer: Insights into Sources, Chemistry, and Interaction with Meteorology[ J], Environmental Science & Technology, 55, 8, pp. 4542-4552, (2021)
  • [7] Liu Y S, Tang G Q, Zhou L B, Et al., Mixing layer transport flux of particulate matter in Beijing, China, Atmospheric Chemistry and Physics, 19, 14, pp. 9531-9540, (2019)
  • [8] Liu Y S, Tang G Q, Wang M, Et al., Impact of residual layer transport on air pollution in Beijing, China, Environmental Pollution, 271, (2020)
  • [9] Wang H, Xu J Y, Zhang M, Et al., A study of the meteorological causes of a prolonged and severe haze episode in January 2013 over central-eastern China, Atmospheric Environment, 98, pp. 146-157, (2014)
  • [10] Chen H P, Wang H J., Haze days in North China and the associated atmospheric circulations based on daily visibility data from 1960 to 2012, Journal of Geophysical Research, 120, 12, pp. 5895-5909, (2015)