Contents and Forms of Phosphorous in the Municipal Sewage Sludge of China

被引:9
|
作者
Wang C. [1 ]
Liu Q.-W. [2 ]
Zhi Y. [2 ]
Cheng L. [1 ]
Wang N. [1 ]
Li C.-D. [1 ]
Mao Y.-X. [1 ]
机构
[1] School of Resources and Environment, Henan Polytechnic University, Jiaozuo
[2] Jiaozuo Environmental Monitoring Station, Jiaozuo
来源
Huanjing Kexue/Environmental Science | 2019年 / 40卷 / 04期
关键词
Bioavailable phosphorus; Municipal sludge; Occurrence forms; Phosphorus; Sludge disposal;
D O I
10.13227/j.hjkx.201809078
中图分类号
学科分类号
摘要
Municipal sludge samples (SS) were collected from 46 cities in China in 2016. The forms in which phosphorus occurred in the SS were evaluated using the Standards, Measurements and Testing (SMT) Program. The results showed that the average contents of total phosphorus (TP), inorganic phosphorus (IP), non-apatite inorganic phosphorus (NAIP), apatite phosphorus (AP), organic phosphorus (OP), and bioavailable phosphorus (NAIP+OP) in the SS were (17.32±5.13), (11.71±4.01), (9.18±3.44), (3.03±2.74), (4.54±4.23), and (13.72±4.36)g•kg-1, respectively. IP was the main form of phosphorus in the SS, accounting for more than 60% of the TP content. NAIP was the main form of IP, accounting for more than 66% of the IP content. There was a highly significant positive correlation between TP and bioavailable phosphorus in the SS (r=0.942, P<0.01), and bioavailable phosphorus accounted for 66.8%-96.1% of the TP content. The contents of phosphorus in the SS and the amounts of phosphorus discharged via SS disposal showed a decreasing trend from the east to the west of China. In 2016, the amount of phosphorus discharged into the environment via SS disposal amounted to 1.04×105 tons, of which 1.95×104 t entered the soil through SS land application, 4.69×104 t entered landfill sites, 1.47×104 t entered building materials, 2.34×104 t ended up in incineration ash, and 4.50 t were directly dumped or discarded. The phosphorus content of the SS of China presented a temporal trend of first increasing and then decreasing. © 2019, Science Press. All right reserved.
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页码:1922 / 1930
页数:8
相关论文
共 42 条
  • [1] Qiao X.L., Luo L.M., Wu S.C., Land use of sewage sludge and its environmental impact, Soils, 32, 2, pp. 79-85, (2000)
  • [2] O'Connor G.A., Sarkar D., Brinton S.R., Et al., Phytoavailability of biosolids phosphorus, Journal of Environmental Quality, 33, 2, pp. 703-712, (2004)
  • [3] Medeiros J.G., Cid B.P., Gomez E.F., Analytical phosphorus fractionation in sewage sludge and sediment samples, Analytical and Bioanalytical Chemistry, 381, 4, pp. 873-878, (2005)
  • [4] Wang C., Feng S.L., Wang P.F., Et al., Distribution of phosphorus fractions and bio-available phosphorus forms and their relationships in sewage sludge, Environmental Science, 29, 6, pp. 1593-1597, (2008)
  • [5] Shen X.L., Zhou Z., Ren W.C., Et al., Fractionation and bioavailability of phosphorus in sludge from municipal wastewater treatment plants, Chinese Journal of Environmental Engineering, 10, 3, pp. 1200-1204, (2016)
  • [6] Wang N., Liu Q.W., Zhi Y., Et al., Spatial and temporal variation of mercury in municipal sewage sludge in China, Environmental Science, 39, 5, pp. 2296-2305, (2018)
  • [7] Ruban V., Lopez-Sanchez J.F., Pardo P., Et al., Harmonized protocol and certified reference material for the determination of extractable contents of phosphorus in freshwater sediments-A synthesis of recent works, Fresenius' Journal of Analytical Chemistry, 370, 2-3, pp. 224-228, (2001)
  • [8] Ruban V., Lopez-Sanchez J.F., Pardo P., Et al., Selection and evaluation of sequential extraction procedures for the determination of phosphorus forms in lake sediment, Journal of Environmental Monitoring, 1, 1, pp. 51-56, (1999)
  • [9] Li Y.X., Chen T.B., Luo W., Et al., Contents of organic matter and major nutrients and the ecological effect related to land application of sewage sludge in China, Acta Ecologica Sinica, 23, 11, pp. 2464-2474, (2003)
  • [10] Li G.B., Yin C.Q., Lin Y.B., Et al., Artifical improvement of soil fertility in a regraded forest ecosystem by using municipal sewage sludge, Chinese Journal of Applied Ecology, 13, 2, pp. 159-162, (2002)