Occurrence, Input, and Seasonal Variations of Poly-and Perfluoroalkyl Substances (PFASs) in Rivers and Drain Outlets from the Dalian Coastal Area, China

被引:0
|
作者
Chen H. [1 ]
Han J.-B. [1 ]
Zhang C. [1 ]
Cheng J.-Y. [1 ]
机构
[1] Key Laboratory of Coastal Ecology and Environment of State Oceanic Administration, National Marine Environmental Monitoring Center, Dalian
来源
Huanjing Kexue/Environmental Science | 2019年 / 40卷 / 05期
关键词
Composition; Input; Poly-and perfluoroalkyl substances (PFASs); Season variation; Source;
D O I
10.13227/j.hjkx.201810132
中图分类号
学科分类号
摘要
Concentrations of 19 PFASs (poly-and perfluoroalkyl substances) in riverwater, coastal wastewater, and effluents from wastewater treatment plants (WWTPs) directly discharged into the Dalian coastal area were measured and their inputs were calculated accordingly. For riverwater samples, the total PFAS concentration ranged from 9.85 to 757 ng•L-1, with a median of 74.7 ng•L-1. For drain outlets, the total PFAS concentration in wastewater ranged from 9.19 to 801 ng•L-1, with a median of 29.5 ng•L-1. PFOS and PFOA were the dominant contributors for the PFASs in both riverwater and wastewater samples in this study. The total PFASs concentration in the industrial wastewater samples collected during the winter were found to be significantly higher than those collected in the summer. However, no seasonal variation was found for other samples. The total PFAS input into the Dalian coastal area was calculated to be 44.7 kg•a-1. The detection frequencies of Cl-PFESAs were low, and no 8:2Cl-PFESA was detected in all collected samples. © 2019, Science Press. All right reserved.
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页码:2115 / 2121
页数:6
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  • [1] Buck R.C., Franklin J., Berger U., Et al., Perfluoroalkyl and polyfluoroalkyl substances in the environment: terminology, classification, and origins, Integrated Environmental Assessment and Management, 7, 4, pp. 513-541, (2011)
  • [2] Bowman J.S., Fluorotechnology is critical to modern life: the fluoroCouncil counterpoint to the madrid statement, Environmental Health Perspective, 123, 5, pp. A112-A113, (2015)
  • [3] Benskin J.P., Phillips V., St. Louis V.L., Et al., Source Elucidation of Perfluorinated Carboxylic Acids in Remote Alpine Lake Sediment cores, Environmental Science & Technology, 45, 17, pp. 7188-7194, (2011)
  • [4] Butt C.M., Berger U., Bossi R., Et al., Levels and trends of poly-and perfluorinated compounds in the Arctic environment, Science of the Total Environment, 408, 15, pp. 2936-2965, (2010)
  • [5] Campo J., Lorenzo M., Perez F., Et al., Analysis of the presence of perfluoroalkyl substances in water, sediment and biota of the Jucar River (E Spain). Sources, Partitioning and Relationships with Water Physical characteristics, Environmental Research, 147, pp. 503-512, (2016)
  • [6] Castiglioni S., Valsecchi S., Polesello S., Et al., Sources and fate of perfluorinated compounds in the aqueous environment and in drinking water of a highly urbanized and industrialized area in Italy, Journal of Hazardous Materials, 282, pp. 51-60, (2015)
  • [7] Karrman A., Ericson I., van Bavel B., Et al., Exposure of perfluorinated chemicals through lactation: levels of matched human milk and serum and a temporal trend, 1996-2004, in Sweden, Environmental Health Perspective, 115, 2, pp. 226-230, (2006)
  • [8] Giesy J.P., Kannan K., Global distribution of perfluorooctane sulfonate in wildlife, Environmental Science & Technology, 35, 7, pp. 1339-1342, (2001)
  • [9] Lau C., Anitole K., Hodes C., Et al., Perfluoroalkyl acids: a review of monitoring and toxicological findings, Toxicological Sciences, 99, 2, pp. 366-394, (2007)
  • [10] Meng D., Wang X., Wang S.S., Et al., Review on combined toxicity of typical heavy metals and perfluorinated compounds in water environment on aquatic organisms, Asian Journal of Ecotoxicology, 13, 2, pp. 13-22, (2018)