Size Distribution of Particulate Chemical Components in Nanjing Jiangbei New Area

被引:0
|
作者
Zhang Y.-X. [1 ]
Yu X.-N. [1 ]
Liu S.-J. [1 ]
An J.-L. [1 ]
Zhang C. [1 ]
机构
[1] Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Collaborative Innovation Center on Forecasting and Evaluation of Meteorological Disasters, Nanjing University of Information Science and Technology, Nanjing
来源
Huanjing Kexue/Environmental Science | 2020年 / 41卷 / 11期
关键词
Elemental carbon (EC); Organic carbon (OC); Particle size distribution; Particulate matter; Seasonal variation; Water-soluble ions;
D O I
10.13227/j.hjkx.202004213
中图分类号
学科分类号
摘要
In order to explore the pollution characteristics of the chemical components of atmospheric particulate matter in Nanjing Jiangbei New Area, size-resolved samples were collected from 2013 to 2014. The size distribution and seasonal variation of the chemical components of the particles were studied. The results showed that the total concentration of nine water-soluble ions in fine particles was higher in autumn and winter than in spring and summer, while the concentration of coarse particles was highest in winter. The ratio of NO3-/SO42- for the fine particles in winter was slightly higher than in the other three seasons, and lowest in the coarse particles. The trend of particle size distribution in spring, summer and autumn was consistent. The distribution of water-soluble ions was bimodal, and NO3- peaked at 0.65- 1.1μm in all four seasons. The peak radius of SO42- in the fine particles in summer and autumn was 0.43- 0.65μm, and the peak value in winter moved towards the coarser particles, while Na+ and Cl- mainly existed in the coarse particles. The charge equivalent of anion and anion indicated that the coarse and fine particles were alkaline and weakly alkaline, respectively. Organic carbon (OC) and elemental carbon (EC) mainly existed in the fine particles, with a bimodal distribution. The secondary organic carbon (SOC) in the fine particles in autumn and winter was significantly higher than in spring and summer. The ratio method further indicated that the carbonaceous component of the particulate matter in Nanjing Jiangbei New Area is mainly from the emissions of coal and biomass combustion, and vehicle exhaust. © 2020, Science Press. All right reserved.
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页码:4803 / 4812
页数:9
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