Fabrication of stainless steel mesh supported zeolite Al-beta coatings for oil/water separation

被引:0
|
作者
Shang X. [1 ]
Zhang B. [1 ]
Li Y. [1 ]
机构
[1] State Key Laboratory of Chemical Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin
来源
Huagong Xuebao/CIESC Journal | 2019年 / 70卷 / 10期
关键词
Film; Oil/water separation; Stability; Stainless steel mesh; Superhydrophilic; Surface; Underwater superhydrophobic; Zeolite Al-beta;
D O I
10.11949/0438-1157.20190355
中图分类号
学科分类号
摘要
The zeolite Al-beta coating was fabricated on the stainless steel mesh by secondary growth method. Scanning electron microscopy (SEM), X-ray diffraction (XRD) and contact angle (CA) measurements were used to characterize the zeolite Al-beta coatings. The cross-linked zeolite Al-beta crystals with spherical morphology on the stainless steel mesh constituted a micro/nanoscale hierarchical structure. The as-synthesized stainless steel mesh supported zeolite Al-beta coatings exhibited superhydrophilic and underwater superoleophobic characteristics. The stainless steel mesh supported zeolite Al-beta coating was applied to the separation of various oil/water mixtures. It could maintain the high separation efficiency above 97.1% after 100 separation cycles. The stability of zeolite Al-beta coatings was checked by using corrosive and ultrasonic treatments. The treated stainless steel mesh supported zeolite Al-beta coatings exhibited almost the same surface morphologies and separation efficiencies as the untreated sample. In addition, the zeolite Al-beta coating displayed a strong attachment to the stainless steel mesh surface. Self-cleaning stainless steel mesh supported zeolite Al-beta coatings with superior durability and stability would show great application potentials in actual oil/water separation processes. © All Right Reserved.
引用
收藏
页码:3994 / 4001
页数:7
相关论文
共 31 条
  • [1] Chan Y.J., Chong M.F., Law C.L., Et al., A review on anaerobic-aerobic treatment of industrial and municipal wastewater, Chemical Engineering Journal, 155, 1, pp. 1-18, (2009)
  • [2] Singh V., Purkait M.K., Das C., Cross-flow microfiltration of industrial oily wastewater: experimental and theoretical consideration, Separation Science and Technology, 46, 8, pp. 1213-1223, (2011)
  • [3] Xue Z.X., Cao Y.Z., Liu N., Et al., Special wettable materials for oil/water separation, Journal of Materials Chemistry A, 2, 8, pp. 2445-2460, (2014)
  • [4] Ma Q.L., Cheng H.F., Fane A.G., Et al., Recent development of advanced materials with special wettability for selective oil/water separation, Small, 12, 16, pp. 2186-2202, (2016)
  • [5] Yuan T., Chen Z., Zhou X.H., Et al., Coated mesh film based on superhydrophilic and superoleophobic principle and its application in oil-water separation, CIESC Journal, 65, 6, pp. 1943-1951, (2014)
  • [6] Dunderdale G.J., England M.W., Sato T., Et al., Programmable oil/water separation meshes: water or oil selectivity using contact angle hysteresis, Macromolecular Materials and Engineering, 301, 9, pp. 1032-1036, (2016)
  • [7] Xiong L., Guo W., Alameda B.M., Et al., Rational design of superhydrophilic/superoleophobic surfaces for oil-water separation via thiol-acrylate photopolymerization, ACS Omega, 3, 8, pp. 10278-10285, (2018)
  • [8] Huang K.T., Yeh S.B., Huang C.J., Surface modification for superhydrophilicity and underwater superoleophobicity: applications in antifog, underwater self-cleaning, and oil-water separation, ACS Applied Materials & Interfaces, 7, 38, pp. 21021-21029, (2015)
  • [9] Chen X.L., Zhai Y.D., Han X., Et al., Surface chemistry-dominated underwater superoleophobic mesh with mussel-inspired zwitterionic coatings for oil/water separation and self-cleaning, Applied Surface Science, 483, pp. 399-408, (2019)
  • [10] Liu J., Li P., Chen L., Et al., Superhydrophilic and underwater superoleophobic modified chitosan-coated mesh for oil/water separation, Surface and Coatings Technology, 307, pp. 171-176, (2016)