Carbon quantum dots modified semiconductor composite photocatalysts for degradation of organic pollutants in water

被引:0
|
作者
Zhang P. [1 ]
Ding S. [1 ]
Gao J. [1 ]
Zhao M. [1 ]
Yu H. [1 ]
Liu Y. [1 ]
Gu L. [1 ]
机构
[1] School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai
关键词
carbon quantum dots (CQDs); composites; degradation; organic pollutants; photocatalyst; semiconductor;
D O I
10.16085/j.issn.1000-6613.2022-2044
中图分类号
学科分类号
摘要
The primary causes of the low efficiency and limited use of conventional photocatalysts in the degradation of organic pollutants in water are the low effective utilisation of visible light and the fast recombination rate of photogenerated charge carrier. Carbon quantum dots (CQDs), a novel nano-zero-dimensional material that modifies semiconductor photocatalysts, can inhibit the recombination of photogenerated carriers, speed up the separation and transfer of carriers, improve the spectral response range, improve the performance of adsorption, promote the reduction of transition metals in the indirect oxidation process and effectively enhance the photocatalytic degradation of organic pollutants in water. This paper reviewed the application of CQDs modified semiconductor composite photocatalyst materials in the degradation of various organic pollutants in water. It focused on the synthesis strategy of CQDs and its modified semiconductor composite photocatalyst materials as well as the enhancement of CQDs in multiphase photocatalytic systems. Furthermore, a brief description was given of the effects of the photocatalytic experimental parameters and the modification of CQDs on the photocatalytic reaction activity. Finally, this paper summarized the unresolved issues during the development of CQDs modified semiconductor composite photocatalysts and gave an outlook on the future development direction. © 2023 Chemical Industry Press. All rights reserved.
引用
收藏
页码:5487 / 5500
页数:13
相关论文
共 99 条
  • [1] SHUI Boyang, SONG Xiaosan, FAN Wenjiang, Research progress and challenges of photocatalytic technology in water treatment, Chemical Industry and Engineering Progress, 40, pp. 356-363, (2021)
  • [2] MEI Aoxue, XL Zijun, WANG Xiyuan, Et al., Photocatalytic materials modified with carbon quantum dots for the degradation of organic pollutants under visible light: A review, Environmental Research, 214, (2022)
  • [3] XU Zheng, SHI Weilong, SHI Yuxing, Et al., Carbon dots as solid-state electron mediator and electron acceptor in S-scheme heterojunction for boosted photocatalytic hydrogen evolutional, Applied Surface Science, 595, (2022)
  • [4] XU Xiaoyou, Robert Ray, GU Yunlong, Et al., Electrophoretic analysis and purification of fluorescent single-walled carbon nanotube fragments, Journal of the American Chemical Society, 126, 40, pp. 12736-12737, (2004)
  • [5] PIRSAHEB Meghdad, ASADI Anvar, SILLANPAA Mika, Et al., Application of carbon quantum dots to increase the activity of conventional photocatalysts: A systematic review, Journal of Molecular Liquids, 271, pp. 857-871, (2018)
  • [6] HAN Mei, ZHL Shoujun, LU Siyu, Et al., Recent progress on the photocatalysis of carbon dots: Classification, mechanism and applications, Nano Today, 19, pp. 201-218, (2018)
  • [7] VELUMANI Arun, SENGODAN Prabhu, ARUMUGAM Priyadharsan, Et al., Carbon quantum dots supported ZnO sphere based photocatalyst for dye degradation application, Current Applied Physics, 20, 10, pp. 1176-1184, (2020)
  • [8] MIAO Xuli, YUE Xiaoyang, JI Zhenyuan, Et al., Nitrogen-doped carbon dots decorated on g-C3N4/Ag3PO4 photocatalyst with improved visible light photocatalytic activity and mechanism insight, Applied Catalysis B: Environmental, 227, pp. 459-469, (2018)
  • [9] ZHOU Qin, HUANG Weiya, XU Chong, Et al., Novel hierarchical carbon quantum dots-dec orated BiOCl nanosheet/carbonized eggshell membrane composites for improved removal of organic contaminants from water via synergistic adsorption and photocatalysis, Chemical Engineering Journal, 420, (2021)
  • [10] WANG Yajun, ZHANG Wencan, LI Yuming, Et al., Research progress of carbon dots in photocatalytic hydrogen production, Chemical Industry and Engineering Progress, 40, 6, pp. 2952-2961, (2021)