Stress-Induced Martensitic Transformation in Na3YCl6

被引：0

作者：

Miura, Akira ^{[1
]}

Muraoka, Koki ^{[2
]}

Maki, Kotaro ^{[3
]}

Kawaguchi, Saori ^{[4
]}

Hikima, Kazuhiro ^{[5
]}

Muto, Hiroyuki ^{[5
,6
]}

Matsuda, Atsunori ^{[5
]}

Yamane, Ichiro ^{[3
]}

Shimada, Toshihiro ^{[1
]}

Ito, Hiroaki ^{[3
]}

Mizuguchi, Yoshikazu ^{[7
]}

Moriyoshi, Chikako ^{[8
]}

Nakajima, Hiroshi ^{[9
]}

Mori, Shigeo ^{[9
]}

Oike, Hiroshi ^{[10
]}

Nakayama, Akira ^{[2
]}

Sun, Wenhao ^{[11
]}

Rosero-Navarro, Nataly Carolina ^{[1
,12
]}

Tadanaga, Kiyoharu ^{[1
]}

机构：

[1] Hokkaido Univ, Fac Engn, Sapporo, Hokkaido 0608628, Japan

[2] Univ Tokyo, Dept Chem Syst Engn, Tokyo 1138656, Japan

[3] Hokkaido Univ, Grad Sch Chem Sci & Engn, Sapporo, Hokkaido 0608628, Japan

[4] Japan Synchrotron Radiat Res Inst, Sayo, Hyogo 6795198, Japan

[5] Toyohashi Univ Technol, Dept Elect & Elect Informat Engn, Toyohashi, Aichi 4418580, Japan

[6] Toyohashi Univ Technol, Inst Liberal Arts & Sci, Toyohashi, Aichi 4418580, Japan

[7] Tokyo Metropolitan Univ, Dept Phys, Tokyo 1920397, Japan

[8] Hiroshima Univ, Grad Sch Adv Sci & Engn, Higashihiroshima 7398526, Japan

[9] Osaka Metropolitan Univ, Grad Sch Engn, Dept Mat Sci, Osaka 5998531, Japan

[10] Japan Sci & Technol Agcy, PRESTO, Kawaguchi, Saitama 3320012, Japan

[11] Univ Michigan, Dept Mat Sci, Ann Arbor, MI 48109 USA

[12] CSIC, Inst Ceram & Vidrio, Madrid 28049, Spain

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2024年 / 146卷 / 36期

关键词：

ROOM-TEMPERATURE; PRESSURE; MODULUS; ZRO2;

D O I：

10.1021/jacs.4c09476

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Martensitic transformation with volume expansion plays a crucial role in enhancing the mechanical properties of steel and partially stabilized zirconia. We believe that a similar concept could be applied to unexplored nonoxide materials. Herein, we report the stress-induced martensitic transformation of monoclinic Na3YCl6 with an similar to 3.4% expansion. In situ synchrotron X-ray diffraction and atomistic simulations showed that anisotropic crystallographic transformation from monoclinic to rhombohedral Na3YCl6 occurs exclusively under uniaxial pressure; no effect is observed under hydrostatic pressure conditions. The uniaxially pressed powder compact of monoclinic Na3YCl6 showed a large indentation impression and low Young's modulus, in contrast to its high bulk modulus, suggesting that these unique mechanical properties are induced by the martensitic transformation.

引用

页码：25263 / 25269

页数：7

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