Highly stable and bright CsPbI3 nanocrystal red emitters based on color-conversion from InGaN-based blue light-emitting diodes

被引:1
|
作者
Yokota, Daisuke [1 ]
Abe, Haruka [2 ]
Saito, Shingo [1 ]
Yanagihashi, Kento [2 ]
Chiba, Takayuki [2 ]
Oto, Takao [1 ]
机构
[1] Yamagata Univ, Dept Informat & Elect, Yonezawa, Yamagata 9928510, Japan
[2] Yamagata Univ, Dept Organ Mat Sci, Yonezawa, Yamagata 9928510, Japan
关键词
EXTERNAL QUANTUM EFFICIENCY; HALIDE PEROVSKITES CSPBX3; ANION-EXCHANGE; STABILITY; BR; CL;
D O I
10.1063/5.0227291
中图分类号
O59 [应用物理学];
学科分类号
摘要
Toward the super-smart society, next-generation display technologies with ultra-small size and high resolution are required. MicroLEDs are promising key technologies for next-generation full-color displays, and the external quantum efficiency in the red region should be improved. To improve red emission efficiency, we propose color-conversion red emitters combined with blue InGaN LEDs and lead-halide perovskite nanocrystals (PNCs) by using a coating process. We improved the stability of PNCs under photoexcitation by dispersing them in a methacrylate-based polymer binder, probably because of the suppressed ligand desorption and nonradiative surface recombination process. PNC films were bonded onto a blue InGaN LED to fabricate a color-conversion LED, demonstrating almost complete red conversion with higher optical performance (power density: 3.5 mW/cm(2); luminance: 1.9 x 10(3) cd/m(2)) at a high current density (270 mW/cm(2)). This performance was achieved while maintaining the same level of external quantum efficiency (26.2%) and device lifetime (103 h) as those reported for the current PNC red LEDs. Therefore, the color-conversion LED may be a milestone in improving the device performance over the entire visible region and realizing low-cost microLED applications.
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页数:6
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