Source-specific ecological risk analysis and critical source identification of heavy metal(loid)s in the soil of typical abandoned coal mining area

被引:0
|
作者
Zhao, Jiyang [1 ]
Cao, Chengying [1 ]
Chen, Xing [1 ,2 ]
Zhang, Wanyu
Ma, Tianqi [1 ]
Irfan, Muhammad [1 ]
Zheng, Liugen [1 ]
机构
[1] Anhui Univ, Sch Resources & Environm Engn, Anhui Prov Engn Lab Mine Ecol Remediat, Hefei 230601, Peoples R China
[2] Anhui Jianzhu Univ, Sch Environm & Energy, Hefei, Peoples R China
基金
中国国家自然科学基金;
关键词
Coal mining; Heavy metal(loid)s; APCS-MLR; Source analysis; Ecological risk; SOURCE APPORTIONMENT; METALS;
D O I
10.1016/j.scitotenv.2024.174506
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Long-term coal mining activities in abandoned coal mining areas have resulted in the migration of large quantities of heavy metals into the surrounding soil environment, posing a threat to the regional ecological environment. This study focuses on the surface soil collected from a typical abandoned coal mining area. Methods such as the pollution index (PI) and potential ecological risk index (RI) were used to comprehensively evaluate the pollution levels and ecological risks of soil heavy metals. Geostatistical analysis and the APCS-MLR model were used to quantify the sources of soil heavy metals, and Nemerow integrated ecological risk (NIRI) model was coupled to apportion the ecological risks from different pollution sources. The results indicate that the average concentrations of Cd, As, and Zn are 4.58, 2.44, and 1.67 times the soil background values, respectively, while the concentrations of other heavy metals are below the soil background values. The soil of study area is strongly polluted by heavy metals, with the pollution level and ecological risk of Cd being significantly higher than those of other heavy metals. The NIRI calculation results show that the overall comprehensive ecological risk level is considerable, with sample points classified as relatively considerable, moderate, and low at 60.53 %, 36.84 %, and 2.63 %, respectively. The sources of soil heavy metals can be categorized into four types: traffic activities, natural sources, coal gangue accumulation, and a combined source of coal mining and agricultural activities, with contribution rates of 35.3 %, 36.1 %, 19.5 %, and 9.1 %, respectively. The specific source ecological risk assessment results indicate that coal gangue accumulation contributes the most to ecological risk (36.4 %) , should be prioritized for pollution control, with Cd being the priority control element for ecological risk. The findings provide theoretical support for the refined management of soil heavy metal pollution in abandoned coal mining areas.
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页数:11
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