Ytterbium-doping contribution to the overall dielectric and electrical properties of (Sr, Ba)Bi2Ta2O9 ceramics

被引:0
|
作者
Afqir, Mohamed [1 ]
Fasquelle, Didier [2 ]
Tachafine, Amina [2 ]
Meng, Yingzhi [3 ]
Elaatmani, Mohamed [1 ]
Zegzouti, Abdelouahad [1 ]
Daoud, Mohamed [1 ]
机构
[1] Univ Cadi Ayyad, Fac Sci Semlalia, Lab Sci Mat & Optimisat Proc, Marrakech, Morocco
[2] Univ Littoral Cote dOpale, Unite Dynam & Struct Mat Mol, Calais, France
[3] Guilin Univ Technol, Guilin 541006, Peoples R China
关键词
Dielectric; Conductivity; Electrical modulus; Sintering; POLARIZATION PROPERTIES; MODIFIED SRBI2TA2O9; RELAXATION;
D O I
10.1007/s41779-024-01068-w
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
In this work, Yb-doped Sr0.95Ba0.05Bi2Ta2O9 powders were synthesized by the citric acid-assisted method. The prepared powders were uniaxially pressed and sintered at different temperatures. Structure, morphology, and dielectric properties were investigated. The use of either a 1200 degrees C sintering temperature or motifs for a reduction tan delta purpose. The results showed that Yb has not caused a significant change in dielectric properties at low temperatures, thus indicating its ability to reduce dielectric loss smoothly. At high temperatures, the introduction of ytterbium elements could reduce both Curie temperature and conductivity. According to Jonscher's universal power law, the correlated barrier-hopping (CBH) model describes the AC conductivity mechanism. However, the non-overlapping small polaron tunneling (NSPT) model may be used to show that this is only possible at a specific temperature. The Arrhenius law and the CBH module provide estimates of the various energy barriers that space charges should overcome; however, these barriers get higher as the dopant concentration rises.
引用
收藏
页码:1601 / 1609
页数:9
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