Continuous Direct Air Capture and Electrochemical Conversion of CO2 and H2O into Ethylene and Oxygen in a Solid Electrolyte Reactor

被引:0
|
作者
Li, Michelle B. [1 ]
Li, Michael [1 ]
Luo, Feirong [1 ]
Zhou, Lili [1 ]
Li, Huaping [1 ]
机构
[1] Chemelectron LLC, Inglewood, CA 90301 USA
关键词
Ethylene;
D O I
10.1021/acs.energyfuels.4c01309
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Direct air capture (DAC) and conversion of carbon dioxide into valuable chemicals is an eco-sustainable solution to curb the urgent climate crisis. This communication demonstrates a practical and scalable solid electrolyte electrochemical cell that can directly uptake CO2 and H2O from air and continuously convert them into basic petrochemical ethylene and oxygen with extremely low voltage potential of 0.6 V and 1 A current. This DAC solid electrolyte reactor can produce approximate 70 mg of ethylene in 1 h, with about 80% energy efficiency, and remain in a lower temperature.
引用
收藏
页码:10390 / 10393
页数:4
相关论文
共 50 条
  • [1] Electrochemical Conversion of CO2 from Direct Air Capture Solutions
    Gutierrez-Sanchez, Oriol
    de Mot, Bert
    Daems, Nick
    Bulut, Metin
    Vaes, Jan
    Pant, Deepak
    Breugelmans, Tom
    ENERGY & FUELS, 2022, 36 (21) : 13115 - 13123
  • [2] Solid Oxide Cell Reactor Model for Transient and Stationary Electrochemical H2O and CO2 Conversion Process Studies
    Sedeqi, F.
    Santhanam, S.
    Riegraf, M.
    Riedel, M.
    Heddrich, M. P.
    Ansar, S. A.
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2024, 171 (07)
  • [3] DEVELOPMENT OF A REACTOR FOR CONTINUOUS ELECTROCHEMICAL REDUCTION OF CO2 USING SOLID ELECTROLYTE
    Aeshala, L. M.
    Rahman, S. U.
    Verma, A.
    PROCEEDINGS OF THE ASME 5TH INTERNATIONAL CONFERENCE ON ENERGY SUSTAINABILITY 2011, PTS A-C, 2012, : 1193 - 1199
  • [4] Contributions of CO2, O2, and H2O to the Oxidative Stability of Solid Amine Direct Air Capture Sorbents at Intermediate Temperature
    Guta, Yoseph A.
    Carneiro, Juliana
    Li, Sichi
    Innocenti, Giada
    Pang, Simon H.
    Sakwa-Novak, Miles A.
    Sievers, Carsten
    Jones, Christopher W.
    ACS APPLIED MATERIALS & INTERFACES, 2023, 15 (40) : 46790 - 46802
  • [5] Pyrrolizidines for direct air capture and CO2 conversion
    Hanusch, Jan M.
    Kerschgens, Isabel P.
    Huber, Florian
    Neuburger, Markus
    Gademann, Karl
    CHEMICAL COMMUNICATIONS, 2019, 55 (07) : 949 - 952
  • [6] Electrochemical conversion of H2O/CO2 to fuel in a proton-conducting solid oxide electrolyser
    Wu, Guojian
    Xie, Kui
    Wu, Yucheng
    Yao, Weitang
    Zhou, Jianer
    JOURNAL OF POWER SOURCES, 2013, 232 : 187 - 192
  • [7] Influence of H2O and CO2 Contamination in Air on the Combustion Properties of Ethylene
    Liu Wei-Xiong
    Yang Yang
    Shao Ju-Xiang
    Song Wen-Yan
    Li Xiang-Yuan
    Le Jia-Ling
    ACTA PHYSICO-CHIMICA SINICA, 2009, 25 (08) : 1618 - 1622
  • [8] Modelling a basalt reactor for direct air CO2 capture
    Schwartz, Michael O.
    ENVIRONMENTAL EARTH SCIENCES, 2022, 81 (07)
  • [9] Modelling a basalt reactor for direct air CO2 capture
    Michael O. Schwartz
    Environmental Earth Sciences, 2022, 81
  • [10] Paired electrochemical process for the capture and conversion of CO2 to ethylene carbonate
    Nam, Ki Tae
    Jang, Jun Ho
    NATURE SYNTHESIS, 2024, 3 (07): : 805 - 806