Spray-Coated MoO3 Hole Transport Layer for Inverted Organic Photovoltaics
被引:2
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作者:
Cha, Hou-Chin
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Natl Atom Res Inst, Dept Phys, Taoyuan 32546, TaiwanNatl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Cha, Hou-Chin
[1
]
Li, Chia-Feng
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机构:
Ming Chi Univ Technol, Dept Mat Engn, New Taipei City 24301, Taiwan
Natl Taiwan Univ, Dept Mat Sci & Engn, Taipei 10617, TaiwanNatl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Li, Chia-Feng
[2
,3
]
Chung, Tsui-Yun
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机构:
Natl Atom Res Inst, Dept Phys, Taoyuan 32546, TaiwanNatl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Chung, Tsui-Yun
[1
]
Ma, Wei-Yang
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Natl Atom Res Inst, Dept Phys, Taoyuan 32546, TaiwanNatl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Ma, Wei-Yang
[1
]
Tsao, Cheng-Si
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机构:
Natl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Natl Taiwan Univ, Dept Mat Sci & Engn, Taipei 10617, TaiwanNatl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Tsao, Cheng-Si
[1
,3
]
Huang, Yu-Ching
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机构:
Ming Chi Univ Technol, Dept Mat Engn, New Taipei City 24301, Taiwan
Ming Chi Univ Technol, Organ Elect Res Ctr, New Taipei City 24301, Taiwan
Chang Gung Univ, Coll Engn, Dept Chem & Mat Engn, Taoyuan 33302, TaiwanNatl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
Huang, Yu-Ching
[2
,4
,5
]
机构:
[1] Natl Atom Res Inst, Dept Phys, Taoyuan 32546, Taiwan
[2] Ming Chi Univ Technol, Dept Mat Engn, New Taipei City 24301, Taiwan
This study focuses on the hole transport layer of molybdenum trioxide (MoO3) for inverted bulk heterojunction (BHJ) organic photovoltaics (OPVs), which were fabricated using a combination of a spray coating and low-temperature annealing process as an alternative to the thermal evaporation process. To achieve a good coating quality of the sprayed film, the solvent used for solution-processed MoO3 (S-MoO3) should be well prepared. Isopropanol (IPA) is added to the as-prepared S-MoO3 solution to control its concentration. MoO3 solutions at concentrations of 5 mg/mL and 1 mg/mL were used for the spray coating process. The power conversion efficiency (PCE) depends on the concentration of the MoO3 solution and the spray coating process parameters of the MoO3 film, such as flow flux, spray cycles, and film thickness. The results of devices fabricated from solution-processed MoO3 with various spray fluxes show a lower PCE than that based on thermally evaporated MoO3 (T-MoO3) due to a limiting FF, which gradually increases with decreasing spray cycles. The highest PCE of 2.8% can be achieved with a 1 mg/mL concentration of MoO3 solution at the sprayed flux of 0.2 mL/min sprayed for one cycle. Additionally, S-MoO3 demonstrates excellent stability. Even without any encapsulation, OPVs can retain 90% of their initial PCE after 1300 h in a nitrogen-filled glove box and under ambient air conditions. The stability of OPVs without any encapsulation still has 90% of its initial PCE after 1300 h in a nitrogen-filled glove box and under air conditions. The results represent an evaluation of the feasibility of solution-processed HTL, which could be employed for a large-area mass production method.
机构:
Pusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Kang, Yong-Jin
Lim, Kyounga
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KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Lim, Kyounga
Jung, Sunghoon
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KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Jung, Sunghoon
Kim, Do-Geun
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KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Kim, Do-Geun
Kim, Jong-Kuk
论文数: 0引用数: 0
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KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Kim, Jong-Kuk
Kim, Chang-Su
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机构:
KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Kim, Chang-Su
Kim, Soo H.
论文数: 0引用数: 0
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Pusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
Kim, Soo H.
Kang, Jae-Wook
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KIMS, Dept Mat Proc, Chang Won 641831, South KoreaPusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South Korea
机构:
Sun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R ChinaSun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China
Liu Wei
Liu Guo-Hong
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机构:
Sun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R ChinaSun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China
Liu Guo-Hong
Liu Yong
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机构:
Sun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R ChinaSun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China
Liu Yong
Li Bao-Jun
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机构:
Sun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R ChinaSun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China
Li Bao-Jun
Zhou Xiang
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Sun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R ChinaSun Yat Sen Univ, Sch Phys & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China
机构:
State Key Lab of Optoelectronic Materials and Technologies,School of Physics and Engineering,Sun Yat-Sen UniversityState Key Lab of Optoelectronic Materials and Technologies,School of Physics and Engineering,Sun Yat-Sen University
刘伟
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刘国红
刘勇
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State Key Lab of Optoelectronic Materials and Technologies,School of Physics and Engineering,Sun Yat-Sen UniversityState Key Lab of Optoelectronic Materials and Technologies,School of Physics and Engineering,Sun Yat-Sen University
机构:
Univ Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, Malaysia
Yap, Chi Chin
Jamil, Nursyafikah
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Univ Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, Malaysia
Jamil, Nursyafikah
Rizauddin, Rini Barizah
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Univ Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, Malaysia
Rizauddin, Rini Barizah
Sahabuddin, Mariah Marsya Anwar
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Univ Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, MalaysiaUniv Kebangsaan Malaysia, Fac Sci & Technol, Dept Appl Phys, Ukm Bangi 43600, Selangor, Malaysia
Sahabuddin, Mariah Marsya Anwar
[J].
JURNAL FIZIK MALAYSIA,
2023,
44
(01):
: 10061
-
10070
机构:
KIMS, Dept Surface Technol, Chang Won 641831, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
Kang, Jae-Wook
Kang, Yong-Jin
论文数: 0引用数: 0
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机构:
KIMS, Dept Surface Technol, Chang Won 641831, South Korea
Pusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
Kang, Yong-Jin
Jung, Sunghoon
论文数: 0引用数: 0
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机构:
KIMS, Dept Surface Technol, Chang Won 641831, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
Jung, Sunghoon
Song, Myungkwan
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机构:
KIMS, Dept Surface Technol, Chang Won 641831, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
Song, Myungkwan
Kim, Do-Geun
论文数: 0引用数: 0
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机构:
KIMS, Dept Surface Technol, Chang Won 641831, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
Kim, Do-Geun
Kim, Chang Su
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KIMS, Dept Surface Technol, Chang Won 641831, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
Kim, Chang Su
Kim, Soo H.
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机构:
Pusan Natl Univ, Dept Nanosyst & Nanoproc Engn, Pusan 609735, South KoreaKIMS, Dept Surface Technol, Chang Won 641831, South Korea
机构:
Indian Inst Technol Delhi, Ctr Energy Studies, Photovolta Lab, New Delhi 110016, India
Indian Inst Technol, Dept Mat Sci & Engn, Kanpur 208016, Uttar Pradesh, India
Indian Inst Technol, Samtel Ctr Display Technol, Kanpur 208016, Uttar Pradesh, IndiaIndian Inst Technol Delhi, Ctr Energy Studies, Photovolta Lab, New Delhi 110016, India
Chaturvedi, Neha
Swami, Sanjay Kumar
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Indian Inst Technol Delhi, Ctr Energy Studies, Photovolta Lab, New Delhi 110016, IndiaIndian Inst Technol Delhi, Ctr Energy Studies, Photovolta Lab, New Delhi 110016, India
Swami, Sanjay Kumar
Dutta, Viresh
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Indian Inst Technol Delhi, Ctr Energy Studies, Photovolta Lab, New Delhi 110016, IndiaIndian Inst Technol Delhi, Ctr Energy Studies, Photovolta Lab, New Delhi 110016, India
机构:
Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Lloyd, Matthew T.
Peters, Craig H.
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Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Peters, Craig H.
Garcia, Andres
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Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Garcia, Andres
Kauvar, Isaac V.
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Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Kauvar, Isaac V.
Berry, Joseph J.
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Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Berry, Joseph J.
Reese, Matthew O.
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Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Reese, Matthew O.
McGehee, Michael D.
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Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
McGehee, Michael D.
Ginley, David S.
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Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA
Ginley, David S.
Olson, Dana C.
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Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USANatl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA