Emission Characteristics and Inventory of Volatile Organic Compounds from Cooking in Sichuan Province

被引:0
|
作者
Qian J. [1 ]
Han L. [1 ]
Chen J.-H. [1 ,2 ]
Wang B. [3 ]
Jiang T. [1 ]
Xu C.-X. [1 ]
Li Y.-J. [1 ]
Wang C.-H. [1 ]
Wang B. [3 ]
机构
[1] Sichuan Academy of Environmental Sciences, Chengdu
[2] School of Environment, Tsinghua University, Beijing
[3] School of Architecture and Environment, Sichuan University, Chengdu
来源
Huanjing Kexue/Environmental Science | 2022年 / 43卷 / 03期
关键词
Cooking; Emission factor; Emission inventory; NMHCs; Sichuan Province; Source profile; Volatile organic compounds (VOCs);
D O I
10.13227/j.hjkx.202104182
中图分类号
学科分类号
摘要
NMHCs concentrations and VOCs components were sampled from 12 typical catering units in Sichuan Province. Combined with literature data, the cooking source profile containing 117 VOCs was established comprehensively, and the NMHCs emission factors were obtained. Based on the bottom-up research method, the volatile organic compounds emission inventory of cooking sources in Sichuan Province was established. The results showed that the oxygen and alkane groups were the most important components for Sichuan cuisine, barbecue, and canteen, and the total proportion of the two groups was greater than 75%. The main VOCs species were ethanol, formaldehyde, ethane, hexanal, ethylene, 1, 3-butadiene, and acrolein. Oxygen-containing components contributed the most to OFP, followed by olefin. The major OFP contributors were formaldehyde, ethylene, ethanol, 1, 3-butadiene, acrolein, hexanal, etc. In 2019, the VOCs emissions and OFP values of cooking sources in Sichuan Province were 32kt and 141kt, respectively, accounting for approximately 5% of the anthropogenic VOCs emissions and OFP values in Sichuan Province. The VOCs emission from cooking may have an important contribution to ozone formation, which means more attention should be paid to cooking. © 2022, Science Press. All right reserved.
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页码:1296 / 1306
页数:10
相关论文
共 26 条
  • [1] Tang X Y, Zhang Y H, Shao M., Atmospheric environmental chemistry, pp. 272-273, (2006)
  • [2] Ye D Q, Liu R Y, Tian J T., Trends of volatile organic compounds emissions and research on policy in China, Environmental Protection, 48, 15, pp. 23-26, (2020)
  • [3] Shao M, Yuan B, Wang M, Et al., Volatile organic compounds in the atmosphere: sources and the roles in atmospheric chemistry, pp. 141-142, (2020)
  • [4] Wang L N, Xiang Z Y, Stevanovic S, Et al., Role of Chinese cooking emissions on ambient air quality and human health, Science of the Total Environment, 589, pp. 173-181, (2017)
  • [5] Zhang D C, Liu J J, Jia L Z, Et al., Speciation of VOCs in the cooking fumes from five edible oils and their corresponding health risk assessments, Atmospheric Environment, 211, pp. 6-17, (2019)
  • [6] Zhou Z H, Deng Y, Lu C W, Et al., Emission inventory and characteristics of volatile organic compounds from anthropogenic sources in Chengdu, Environmental Monitoring in China, 33, 3, pp. 39-48, (2017)
  • [7] Xia S J, Liu Q, Zhao Q Y., Emission inventory of anthropogenically sourced VOCs and its contribution to ozone formation in Jiangsu Province, Environmental Science, 39, 2, pp. 592-599, (2018)
  • [8] Wang C H, Chen J H, Han L, Et al., Seasonal pollution characteristics and analysis of the sources of atmospheric VOCs in Chengdu urban area, Environmental Science, 41, 9, pp. 3951-3960, (2020)
  • [9] Gao Y Q, Wang H L, Xu R Z, Et al., Characterization of volatile organic compounds from cooking emissions, Environmental Science, 40, 4, pp. 1627-1633, (2019)
  • [10] He W Q, Nie L, Tian G, Et al., Study on the chemical compositions of VOCs emitted by cooking oils based on GC-MS, Environmental Science, 34, 12, pp. 4605-4611, (2013)