Properties of nonclassical correlated Stokes-anti-Stokes photon pair in decane

被引：0
|
作者：
de Aguiar Junior, Filomeno S. [1 ,2 ]
Monken, Carlos H. [1 ]
Jorio, Ado [1 ]
机构：
[1] Univ Fed Minas Gerais, Dept Fis ICEx, Ave Antonio Carlos 6627, Belo Horizonte BR-31270901, MG, Brazil
[2] Univ Victoria, Dept Chem, Victoria, BC V8W 2Y2, Canada
来源：
PHYSICAL REVIEW B | 2024年 / 109卷 / 02期
关键词：
RAMAN-SPECTRA;
D O I：
10.1103/PhysRevB.109.024304
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
In this study, the correlated Stokes-anti-Stokes Raman scattering, denominated as the SaS process, is investigated in a decane sample, generalizing for a liquid the results observed in crystalline diamond. The production of SaS photon pairs is observed in both real and virtual processes by measuring nonclassical values of the second-order cross-correlation function g2SaS(0). The correlated Raman spectrum is observed only for Raman shift values below approximately 2900 cm-1, which is equivalent to the highest vibrational mode of the decane molecule. Furthermore, despite the fact that decane is a liquid, the polarization and spatial profile of the SaS process in decane presents the same properties as those observed in diamond.
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页数：7
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