The neutron emission-rate (NER) method for burnup measurement of a spent LWR fuel bundle submerged in water has been studied by focusing on the spatial higher harmonics effects inevitable for the application of a formula based on the one-point reactor model. Verification studies of this method have been made through calculations and simulation experiments using the fresh UO2 fuel-rod bundles of n x n arrays (3 less-than-or-equal-to n less-than-or-equal-to 23, 0.22 less-than-or-equal-to k(eff) less-than-or-equal-to 0.94), and its applicability has been shown for the spent fuel bundle. As a practical example, an actual formula has been given for a spent PWR fuel bundle of 14 x 14 array of 3.5 wt% initial enrichment and cooling time of 1,000 days.