FEMTOSECOND PUMP-PROBE SPECTROSCOPY OF INTERMOLECULAR VIBRATIONS IN MOLECULAR DIMERS

被引：15
|
作者：
TANIMURA, Y [1 ]
MUKAMEL, S [1 ]
机构：
[1] UNIV ROCHESTER,DEPT CHEM,ROCHESTER,NY 14627
来源：
JOURNAL OF CHEMICAL PHYSICS | 1995年 / 103卷 / 05期
关键词：
D O I：
10.1063/1.469722
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The dynamics of intermolecular vibrations in molecular aggregates can be directly monitored by ultrafast spectroscopic techniques. Starting with the third order response function obtained using the path-integral approach, we calculate the pump-probe spectrum of a molecular dimer, taking into account the effects of an intermolecular vibration coupled to the solvent. The various contributions to the signal which represent distinct Liouville space paths are identified and analyzed. (C) 1995 American Institute of Physics.
引用
收藏
页码：1981 / 1984
页数：4
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